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000042723 0247_ $$2DOI$$a10.1029/2003JD003961
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000042723 084__ $$2WoS$$aMeteorology & Atmospheric Sciences
000042723 1001_ $$0P:(DE-HGF)0$$aKulmala, M.$$b0
000042723 245__ $$aOrganic aerosol formation via sulphate cluster activation
000042723 260__ $$aWashington, DC$$bUnion$$c2004
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000042723 440_0 $$06393$$aJournal of Geophysical Research D: Atmospheres$$v109$$x0148-0227$$yD4
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000042723 520__ $$a[ 1] The formation of aerosols, and subsequent cloud condensation nuclei, remains one of the least understood atmospheric processes upon which global climate change critically depends. Under atmospheric conditions, the process of homogeneous nucleation (formation of stable clusters -1 nm in size), and their subsequent growth into new particles (>3 nm), determines the aerosol and cloud nuclei population, yet, hitherto, no theory has elucidated the new particle formation phenomenon in detail. In this study, we present a new theory which provides a mechanistic explanation for new particle formation via activation of stable inorganic clusters by organic vapors. The new nano-particle activation theory is analogous to Kohler theory which describes cloud formation in a supersaturated water vapor field but differs in that it describes the activation of inorganic stable nano-clusters into aerosol particles in a supersaturated organic vapor which initiates spontaneous and rapid growth of clusters. Inclusion of the new theory into aerosol formation models predicts that increases in organic vapor densities lead to even greater increases in particle production, which, in turn, will influence the global radiative cooling effect of atmospheric aerosols.
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000042723 7001_ $$0P:(DE-HGF)0$$aKerminen, V.-M.$$b1
000042723 7001_ $$0P:(DE-Juel1)VDB45939$$aAnttila, T.$$b2$$uFZJ
000042723 7001_ $$0P:(DE-HGF)0$$aLaaksonen, A.$$b3
000042723 7001_ $$0P:(DE-HGF)0$$aO'Dowd, K. A.$$b4
000042723 773__ $$0PERI:(DE-600)2016800-7 $$a10.1029/2003JD003961$$gVol. 109, p. D04205$$pD04205$$q109<D04205$$tJournal of geophysical research / Atmospheres  $$tJournal of Geophysical Research$$v109$$x0148-0227$$y2004
000042723 8567_ $$uhttp://dx.doi.org/10.1029/2003JD003961
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