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@ARTICLE{Hofer:43108,
author = {Hofer, C. and Meyer, R. and Böttger, U. and Waser, R.},
title = {{C}haracterization of {B}a({T}i,{Z}r){O}3 ceramics sintered
under reducing conditions},
journal = {Journal of the European Ceramic Society},
volume = {24},
issn = {0955-2219},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {PreJuSER-43108},
pages = {1473 - 1477},
year = {2004},
note = {Record converted from VDB: 12.11.2012},
abstract = {Over the past few years, lead-free relaxor dielectrics have
become particularly interesting for industrial applications.
Due to the use of low cost base metal electrodes (BME),
reductive sample sintering is required. This contribution
refers to the influence of reducing sintering atmospheres on
the dielectric behaviour of Mn-doped Ba(TixZr1-x)O-3
ceramics with different Zr-contents (x = 0-100 $at.\%).$ It
was studied by impedance spectroscopy in the temperature
range T = -150-300 degreesC and the frequency range f= 5
mHz-10 MHz. For the interpretation of the impedance spectra
we used an equivalent electrical circuit to separate bulk
from grain boundary or electrode contributions,
respectively. It was found that reductive sintering
decreases the maximum dielectric constant by approx. $20\%.$
Further, a T-Curie, shift towards lower temperatures was
observed, In contrast to materials sintered under oxidizing
conditions, reduced sintered samples showed a plateau in the
T-Curie versus Zr-content plot, derived from the Curie-Weiss
behavior of the bulk in the cubic phase. (C) 2003 Elsevier
Ltd. All rights reserved.},
keywords = {J (WoSType)},
cin = {IFF-IEM / CNI},
ddc = {660},
cid = {I:(DE-Juel1)VDB321 / I:(DE-Juel1)VDB381},
pnm = {Materialien, Prozesse und Bauelemente für die Mikro- und
Nanoelektronik},
pid = {G:(DE-Juel1)FUEK252},
shelfmark = {Materials Science, Ceramics},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000189247800113},
doi = {10.1016/S0955-2219(03)00573-9},
url = {https://juser.fz-juelich.de/record/43108},
}