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000053860 0247_ $$2DOI$$a10.1103/PhysRevLett.96.207401
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000053860 084__ $$2WoS$$aPhysics, Multidisciplinary
000053860 1001_ $$0P:(DE-Juel1)130885$$aPersson, B. N. J.$$b0$$uFZJ
000053860 245__ $$aChemical contribution to surface-enhanced Raman scattering
000053860 260__ $$aCollege Park, Md.$$bAPS$$c2006
000053860 300__ $$a207401
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000053860 440_0 $$04925$$aPhysical Review Letters$$v96$$x0031-9007$$y20
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000053860 520__ $$aWe present a new mechanism for the chemical contribution to surface-enhanced Raman scattering (SERS). The theory considers the modulation of the polarizability of a metal nanocluster or a flat metal surface by the vibrational motion of an adsorbed molecule. The modulated polarization of the substrate coupled with the incident light will contribute to the Raman scattering enhancement. We show that for a metal cluster and for a flat metal surface this new chemical contribution may enhance the Raman scattering intensity by a factor of similar to 10(2) and similar to 10(4), respectively. The new SERS process is determined by the electric field parallel to the surface of the metal substrate at the molecular binding site.
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000053860 7001_ $$0P:(DE-HGF)0$$aZhao, K.$$b1
000053860 7001_ $$0P:(DE-HGF)0$$aZhang, Z. Y.$$b2
000053860 773__ $$0PERI:(DE-600)1472655-5$$a10.1103/PhysRevLett.96.207401$$gVol. 96, p. 207401$$p207401$$q96<207401$$tPhysical review letters$$v96$$x0031-9007$$y2006
000053860 8567_ $$uhttp://hdl.handle.net/2128/1456$$uhttp://dx.doi.org/10.1103/PhysRevLett.96.207401
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