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@ARTICLE{Gehlmann:810023,
author = {Gehlmann, Mathias and Aguilera, Irene and Bihlmayer, Gustav
and Mlynczak, Ewa and Eschbach, Markus and Döring, Sven and
Gospodarič, Pika and Cramm, Stefan and Kardynal, Beata and
Plucinski, Lukasz and Blügel, Stefan and Schneider, Claus
M.},
title = {{Q}uasi 2{D} electronic states with high spin-polarization
in centrosymmetric {M}o{S}$_{2}$ bulk crystals},
journal = {Scientific reports},
volume = {6},
issn = {2045-2322},
address = {London},
publisher = {Nature Publishing Group},
reportid = {FZJ-2016-02906},
pages = {26197},
year = {2016},
abstract = {Time reversal dictates that nonmagnetic, centrosymmetric
crystals cannot be spin-polarized as a whole. However, it
has been recently shown that the electronic structure in
these crystals can in fact show regions of high
spin-polarization, as long as it is probed locally in real
and in reciprocal space. In this article we present the
first observation of this type of compensated polarization
in MoS2 bulk crystals. Using spin- and angle-resolved
photoemission spectroscopy (ARPES), we directly observed a
spin-polarization of more than $65\%$ for distinct valleys
in the electronic band structure. By additionally evaluating
the probing depth of our method, we find that these valence
band states at the point in the Brillouin zone are close to
fully polarized for the individual atomic trilayers of MoS2,
which is confirmed by our density functional theory
calculations. Furthermore, we show that this spin-layer
locking leads to the observation of highly spin-polarized
bands in ARPES since these states are almost completely
confined within two dimensions. Our findings prove that
these highly desired properties of MoS2 can be accessed
without thinning it down to the monolayer limit.},
cin = {PGI-6 / PGI-1 / PGI-9 / IAS-1 / JARA-FIT / JARA-HPC},
ddc = {000},
cid = {I:(DE-Juel1)PGI-6-20110106 / I:(DE-Juel1)PGI-1-20110106 /
I:(DE-Juel1)PGI-9-20110106 / I:(DE-Juel1)IAS-1-20090406 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) / 143 -
Controlling Configuration-Based Phenomena (POF3-143) / 522 -
Controlling Spin-Based Phenomena (POF3-522) / Magnetic
Anisotropy of Metallic Layered Systems and Nanostructures
$(jiff13_20131101)$},
pid = {G:(DE-HGF)POF3-142 / G:(DE-HGF)POF3-143 /
G:(DE-HGF)POF3-522 / $G:(DE-Juel1)jiff13_20131101$},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000376857600001},
pubmed = {pmid:27245646},
doi = {10.1038/srep26197},
url = {https://juser.fz-juelich.de/record/810023},
}