Journal Article FZJ-2016-04116

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A novel Ni/ceria-based anode for metal-supported solid oxide fuel cells

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2016
Elsevier New York, NY [u.a.]

Journal of power sources 328, 65-74 () [10.1016/j.jpowsour.2016.07.075]

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Abstract: For optimization of ageing behavior, electrochemical performance, and sulfur tolerance of metal-supported solid oxide fuel cells a new anode concept is introduced, which is based on a Ni/GDC cermet replacing the established Ni/YSZ anodes. In the present work optimized processing parameters compatible with MSC substrates are specified by doing sintering studies on pressed bulk specimen and on real porous anode structures. The electrochemical performance of the Ni/GDC anodes was characterized by means of symmetrical electrolyte supported model-type cells. In this study, three main objectives are pursued. Firstly, the effective technical realization of the Ni/GDC concept is demonstrated. Secondly, the electrochemical behavior of Ni/GDC porous anodes is characterized by impedance spectroscopy and compared with the current standard Ni/YSZ anode. Further, a qualitative comparison of the sulfur poisoning behavior of both anode types is presented. Thirdly, preliminary results of a successful implementation of the Ni/GDC cermet into a metal-supported single cell are presented.

Classification:

Contributing Institute(s):
  1. Werkstoffsynthese und Herstellungsverfahren (IEK-1)
Research Program(s):
  1. 135 - Fuel Cells (POF3-135) (POF3-135)
  2. SOFC - Solid Oxide Fuel Cell (SOFC-20140602) (SOFC-20140602)

Appears in the scientific report 2016
Database coverage:
Medline ; Current Contents - Engineering, Computing and Technology ; Current Contents - Physical, Chemical and Earth Sciences ; IF >= 5 ; JCR ; NCBI Molecular Biology Database ; No Authors Fulltext ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection
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Dokumenttypen > Aufsätze > Zeitschriftenaufsätze
Institutssammlungen > IMD > IMD-2
Workflowsammlungen > Öffentliche Einträge
IEK > IEK-1
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