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005     20220930130107.0
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100 1 _ |0 P:(DE-Juel1)156533
|a Esat, Taner
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245 _ _ |a A chemically driven quantum phase transition in a two-molecule Kondo system
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520 _ _ |a The magnetic properties of nanostructures that consist of a small number of atoms or molecules are typically determined by magnetic exchange interactions. Here, we show that non-magnetic, chemical interactions can have a similarly decisive effect if spin-moment-carrying orbitals extend in space and therefore allow the direct coupling of magnetic properties to wavefunction overlap and the formation of bonding and antibonding orbitals. We demonstrate this for a dimer of metal–molecule complexes on the Au(111) surface. A changing wavefunction overlap between the two monomers drives the surface-adsorbed dimer through a quantum phase transition from an underscreened triplet to a singlet ground state, with one configuration being located extremely close to a quantum critical point.
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|a Lechtenberg, Benedikt
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|a Wagner, Christian
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|a Temirov, Ruslan
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|a Anders, Frithjof B.
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|t Nature physics
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