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000819518 1001_ $$0P:(DE-Juel1)145058$$aTuran, Bugra$$b0$$eCorresponding author
000819518 245__ $$aUpscaling of integrated photoelectrochemical water-splitting devices to large areas
000819518 260__ $$aLondon$$bNature Publishing Group$$c2016
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000819518 520__ $$aPhotoelectrochemical water splitting promises both sustainable energy generation and energy storage in the form of hydrogen. However, the realization of this vision requires laboratory experiments to be engineered into a large-scale technology. Up to now only few concepts for scalable devices have been proposed or realized. Here we introduce and realize a concept which, by design, is scalable to large areas and is compatible with multiple thin-film photovoltaic technologies. The scalability is achieved by continuous repetition of a base unit created by laser processing. The concept allows for independent optimization of photovoltaic and electrochemical part. We demonstrate a fully integrated, wireless device with stable and bias-free operation for 40 h. Furthermore, the concept is scaled to a device area of 64 cm2 comprising 13 base units exhibiting a solar-to-hydrogen efficiency of 3.9%. The concept and its successful realization may be an important contribution towards the large-scale application of artificial photosynthesis.
000819518 536__ $$0G:(DE-HGF)POF3-121$$a121 - Solar cells of the next generation (POF3-121)$$cPOF3-121$$fPOF III$$x0
000819518 536__ $$0G:(DE-Juel1)HITEC-20170406$$aHITEC - Helmholtz Interdisciplinary Doctoral Training in Energy and Climate Research (HITEC) (HITEC-20170406)$$cHITEC-20170406$$x1
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000819518 7001_ $$0P:(DE-Juel1)142337$$aBecker, Jan-Philipp$$b1
000819518 7001_ $$0P:(DE-Juel1)156469$$aUrbain, Félix$$b2
000819518 7001_ $$0P:(DE-Juel1)130238$$aFinger, Friedhelm$$b3$$ufzj
000819518 7001_ $$0P:(DE-Juel1)143905$$aRau, Uwe$$b4$$ufzj
000819518 7001_ $$0P:(DE-Juel1)130246$$aHaas, Stefan$$b5$$ufzj
000819518 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/ncomms12681$$gVol. 7, p. 12681 -$$p12681$$tNature Communications$$v7$$x2041-1723$$y2016
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