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100 1 _ |a Turan, Bugra
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245 _ _ |a Upscaling of integrated photoelectrochemical water-splitting devices to large areas
260 _ _ |a London
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520 _ _ |a Photoelectrochemical water splitting promises both sustainable energy generation and energy storage in the form of hydrogen. However, the realization of this vision requires laboratory experiments to be engineered into a large-scale technology. Up to now only few concepts for scalable devices have been proposed or realized. Here we introduce and realize a concept which, by design, is scalable to large areas and is compatible with multiple thin-film photovoltaic technologies. The scalability is achieved by continuous repetition of a base unit created by laser processing. The concept allows for independent optimization of photovoltaic and electrochemical part. We demonstrate a fully integrated, wireless device with stable and bias-free operation for 40 h. Furthermore, the concept is scaled to a device area of 64 cm2 comprising 13 base units exhibiting a solar-to-hydrogen efficiency of 3.9%. The concept and its successful realization may be an important contribution towards the large-scale application of artificial photosynthesis.
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700 1 _ |a Becker, Jan-Philipp
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700 1 _ |a Urbain, Félix
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700 1 _ |a Finger, Friedhelm
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700 1 _ |a Rau, Uwe
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700 1 _ |a Haas, Stefan
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