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@ARTICLE{Arinicheva:835088,
author = {Arinicheva, Yulia and Popa, Karin and Scheinost, Andreas C.
and Rossberg, André and Dieste-Blanco, Oliver and Raison,
Philippe and Cambriani, Andrea and Somers, Joseph and
Bosbach, Dirk and Neumeier, Stefan},
title = {{S}tructural investigations of ({L}a,{P}u){PO}$_{4}$
monazite solid solutions: {XRD} and {XAFS} study},
journal = {Journal of nuclear materials},
volume = {493},
issn = {0022-3115},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2017-04956},
pages = {404 - 411},
year = {2017},
abstract = {A solid state method was used to synthesize La1-xPuxPO4 (x
= 0.01, 0.05, 0.10, 0.15, (0.5)) solid solutions with
monazite structure. XRD measurements of the compounds with x
= 0.50 revealed the formation of two phases:
(La,Pu)PO4-monazite and a cubic phase (PuO2). Pure-phase
La1-xPuxPO4-monazite solid solutions were obtained for
materials with x = 0.00–0.15 and confirmed by a linear
dependence of the lattice parameters on composition
according to Vegard's law. X-ray absorption spectroscopy
(XAS) analysis at the Pu-LIII and La-LIII edges confirmed
the +III valence state of plutonium in the monazite solid
solutions. The local environment of Pu is PuPO4-like along
the solid solution series, except for the longest fitted
cation-cation distance, which may be an indication of
cluster formation consisting of a few Pu-atoms in the
La-Pu-monazite lattice.},
cin = {IEK-6},
ddc = {530},
cid = {I:(DE-Juel1)IEK-6-20101013},
pnm = {161 - Nuclear Waste Management (POF3-161) / BMBF-02NUK021A
- Verbundprojekt Conditioning: Grundlegende Untersuchungen
zur Immobilisierung langlebiger Radionuklide mittels Einbau
in endlagerrelevante Keramiken; Teilprojekt A
(BMBF-02NUK021A)},
pid = {G:(DE-HGF)POF3-161 / G:(DE-Juel1)BMBF-02NUK021A},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000408044000043},
doi = {10.1016/j.jnucmat.2017.06.034},
url = {https://juser.fz-juelich.de/record/835088},
}