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@ARTICLE{vandenHam:837639,
author = {van den Ham, Evert and Maino, Giulia and Bonneux, Gilles
and Marchal, Wouter and Elen, Ken and Gielis, Sven and
Mattelaer, Felix and Detavernier, Christophe and Notten,
Peter H. L. and Van Bael, Marlies and Hardy, An},
title = {{W}et-{C}hemical {S}ynthesis of 3{D} {S}tacked {T}hin
{F}ilm {M}etal-{O}xides for {A}ll-{S}olid-{S}tate {L}i-{I}on
{B}atteries},
journal = {Materials},
volume = {10},
number = {9},
issn = {1996-1944},
address = {Basel},
publisher = {MDPI},
reportid = {FZJ-2017-06517},
pages = {1072 -},
year = {2017},
abstract = {By ultrasonic spray deposition of precursors, conformal
deposition on 3D surfaces of tungsten oxide (WO3) negative
electrode and amorphous lithium lanthanum titanium oxide
(LLT) solid-electrolyte has been achieved as well as an
all-solid-state half-cell. Electrochemical activity was
achieved of the WO3 layers, annealed at temperatures of 500
°C. Galvanostatic measurements show a volumetric capacity
(415 mAh·cm−3) of the deposited electrode material. In
addition, electrochemical activity was shown for half-cells,
created by coating WO3 with LLT as the solid-state
electrolyte. The electron blocking properties of the LLT
solid-electrolyte was shown by ferrocene reduction. 3D
depositions were done on various micro-sized Si template
structures, showing fully covering coatings of both WO3 and
LLT. Finally, the thermal budget required for WO3 layer
deposition was minimized, which enabled attaining active WO3
on 3D TiN/Si micro-cylinders. A 2.6-fold capacity increase
for the 3D-structured WO3 was shown, with the same current
density per coated area.},
cin = {IEK-9},
ddc = {600},
cid = {I:(DE-Juel1)IEK-9-20110218},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000411506700082},
pubmed = {pmid:28895931},
doi = {10.3390/ma10091072},
url = {https://juser.fz-juelich.de/record/837639},
}