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024 7 _ |a 10.1103/PhysRevB.96.035301
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024 7 _ |a 1094-1622
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024 7 _ |a 2469-9950
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100 1 _ |a Lüpke, Felix
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245 _ _ |a Chalcogenide-based van der Waals epitaxy: Interface conductivity of tellurium on Si(111)
260 _ _ |a Woodbury, NY
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520 _ _ |a We present a combined experimental and theoretical analysis of a Te rich interface layer which represents a template for chalcogenide-based van der Waals epitaxy on Si(111). On a clean Si(111)-(1×1) surface, we find Te to form a Te/Si(111)-(1×1) reconstruction to saturate the substrate bonds. A problem arising is that such an interface layer can potentially be highly conductive, undermining the applicability of the on-top grown films in electric devices. We perform here a detailed structural analysis of the pristine Te termination and present direct measurements of its electrical conductivity by in situ distance-dependent four-probe measurements. The experimental results are analyzed with respect to density functional theory calculations and the implications of the interface termination with respect to the electrical conductivity of chalcogenide-based topological insulator thin films are discussed. In detail, we find a Te/Si(111)-(1×1) interface conductivity of σTe2D=2.6(5)×10−7S/□, which is small compared to the typical conductivity of topological surface states.
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700 1 _ |a Just, Sven
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700 1 _ |a Bihlmayer, Gustav
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700 1 _ |a Lanius, Martin
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700 1 _ |a Luysberg, Martina
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700 1 _ |a Doležal, Jiří
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700 1 _ |a Neumann, Elmar
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700 1 _ |a Cherepanov, Vasily
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700 1 _ |a Ošt'ádal, Ivan
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700 1 _ |a Mussler, Gregor
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700 1 _ |a Grützmacher, Detlev
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700 1 _ |a Voigtländer, Bert
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773 1 8 |a 10.1103/physrevb.96.035301
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773 _ _ |a 10.1103/PhysRevB.96.035301
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Marc 21