Journal Article FZJ-2017-06866

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Impedance of a PEM Fuel Cell Cathode with Nonuniform Ionomer Loading: Analytical and Numerical Study



2017
Elsevier New York, NY [u.a.]

Journal of electroanalytical chemistry 789, 174 - 180 () [10.1016/j.jelechem.2017.02.029]

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Abstract: We report a physics-based model for impedance of the cathode catalyst layer (CCL) with nonuniform Nafion loading in a PEM fuel cell. The general system of equations for the perturbation amplitudes is derived and solved analytically for the cases of either fast oxygen transport, or fast proton transport in the CCL. The expressions for the respective CCL impedances are obtained. In the case of large cell current, we analyse the numerical solutions for the CCL impedance.

Classification:

Contributing Institute(s):
  1. Elektrochemische Verfahrenstechnik (IEK-3)
Research Program(s):
  1. 135 - Fuel Cells (POF3-135) (POF3-135)

Appears in the scientific report 2017
Database coverage:
Medline ; Current Contents - Physical, Chemical and Earth Sciences ; Ebsco Academic Search ; IF < 5 ; JCR ; NationallizenzNationallizenz ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection
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 Record created 2017-10-05, last modified 2024-07-11


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