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000844305 1001_ $$0P:(DE-HGF)0$$aRuckdeschel, Pia$$b0$$eCorresponding author
000844305 245__ $$aThermal transport in binary colloidal glasses: Composition dependence and percolation assessment
000844305 260__ $$aWoodbury, NY$$bInst.$$c2018
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000844305 520__ $$aThe combination of various types of materials is often used to create superior composites that outperform the pure phase components. For any rational design, the thermal conductivity of the composite as a function of the volume fraction of the filler component needs to be known. When approaching the nanoscale, the homogeneous mixture of various components poses an additional challenge. Here, we investigate binary nanocomposite materials based on polymer latex beads and hollow silica nanoparticles. These form randomly mixed colloidal glasses on a sub-μm scale. We focus on the heat transport properties through such binary assembly structures. The thermal conductivity can be well described by the effective medium theory. However, film formation of the soft polymer component leads to phase segregation and a mismatch between existing mixing models. We confirm our experimental data by finite element modeling. This additionally allowed us to assess the onset of thermal transport percolation in such random particulate structures. Our study contributes to a better understanding of thermal transport through heterostructured particulate assemblies.
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000844305 7001_ $$0P:(DE-HGF)0$$aPhilipp, Alexandra$$b1
000844305 7001_ $$0P:(DE-HGF)0$$aKopera, Bernd A. F.$$b2
000844305 7001_ $$0P:(DE-HGF)0$$aBitterlich, Flora$$b3
000844305 7001_ $$0P:(DE-Juel1)172746$$aDulle, Martin$$b4
000844305 7001_ $$0P:(DE-HGF)0$$aPech-May, Nelson W.$$b5
000844305 7001_ $$0P:(DE-HGF)0$$aRetsch, Markus$$b6$$eCorresponding author
000844305 77318 $$2Crossref$$3journal-article$$a10.1103/physreve.97.022612$$bAmerican Physical Society (APS)$$d2018-02-15$$n2$$p022612$$tPhysical Review E$$v97$$x2470-0045$$y2018
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