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000844862 0247_ $$2doi$$a10.5194/acp-18-3147-2018
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000844862 1001_ $$0P:(DE-Juel1)164575$$aStadtler, Scarlet$$b0$$eCorresponding author
000844862 245__ $$aOzone impacts of gas–aerosol uptake in global chemistry transport models
000844862 260__ $$aKatlenburg-Lindau$$bEGU$$c2018
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000844862 520__ $$aThe impact of six heterogeneous gas–aerosol up-take  reactions  on  tropospheric  ozone  and  nitrogen  specieswas studied using two chemical transport models, the Mete-orological Synthesizing Centre-West of the European Moni-toring and Evaluation Programme (EMEP MSC-W) and theEuropean Centre Hamburg general circulation model com-bined  with  versions  of  the  Hamburg  Aerosol  Model  andModel for Ozone and Related chemical Tracers (ECHAM-HAMMOZ). Species undergoing heterogeneous reactions inboth models include N2O5, NO3, NO2, O3, HNO3, and HO2.Since heterogeneous reactions take place at the aerosol sur-face area, the modelled surface area density (Sa) of both mod-els was compared to a satellite product retrieving the surfacearea. This comparison shows a good agreement in global pat-tern and especially the capability of both models to capturethe extreme aerosol loadings in east Asia.The impact of the heterogeneous reactions was evaluatedby the simulation of a reference run containing all hetero-geneous reactions and several sensitivity runs. One reactionwas  turned  off  in  each  sensitivity  run  to  compare  it  withthe reference run. The analysis of the sensitivity runs con-firms that the globally most important heterogeneous reac-tion  is  the  one  of  N2O5.  Nevertheless,  NO2,  HNO3,  andHO2heterogeneous reactions gain relevance particularly ineast  Asia  due  to  the  presence  of  high  NOxconcentrationsand highSain the same region. The heterogeneous reactionof O3itself on dust is of minor relevance compared to theother heterogeneous reactions. The impacts of the N2O5re-actions show strong seasonal variations, with the biggest im-pacts on O3in springtime when photochemical reactions areactive and N2O5levels still high. Evaluation of the modelswith northern hemispheric ozone surface observations yieldsa better agreement of the models with observations in termsof concentration levels, variability, and temporal correlationsat most sites when the heterogeneous reactions are incorpo-rated. Our results are loosely consistent with results from ear-lier studies, although the magnitude of changes induced byN2O5reaction is at the low end of estimates, which seems tofit a trend, whereby the more recent the study the lower theimpacts of these reactions
000844862 536__ $$0G:(DE-HGF)POF3-243$$a243 - Tropospheric trace substances and their transformation processes (POF3-243)$$cPOF3-243$$fPOF III$$x0
000844862 536__ $$0G:(DE-Juel1)jicg23_20151101$$aChemical processes in the troposphere and their impact on climate (jicg23_20151101)$$cjicg23_20151101$$fChemical processes in the troposphere and their impact on climate$$x1
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000844862 7001_ $$00000-0001-9538-3208$$aSimpson, David$$b1$$eCorresponding author
000844862 7001_ $$0P:(DE-Juel1)16212$$aSchröder, Sabine$$b2
000844862 7001_ $$0P:(DE-Juel1)167439$$aTaraborrelli, Domenico$$b3
000844862 7001_ $$0P:(DE-HGF)0$$aBott, Andreas$$b4
000844862 7001_ $$0P:(DE-Juel1)6952$$aSchultz, Martin$$b5
000844862 773__ $$0PERI:(DE-600)2069847-1$$a10.5194/acp-18-3147-2018$$gVol. 18, no. 5, p. 3147 - 3171$$n5$$p3147 - 3171$$tAtmospheric chemistry and physics$$v18$$x1680-7324$$y2018
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