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| 001 | 850872 | ||
| 005 | 20240711085629.0 | ||
| 024 | 7 | _ | |a 10.1016/j.jpowsour.2018.04.059 |2 doi |
| 024 | 7 | _ | |a 0378-7753 |2 ISSN |
| 024 | 7 | _ | |a 1873-2755 |2 ISSN |
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| 100 | 1 | _ | |a Rossbach, Andreas |0 P:(DE-Juel1)171271 |b 0 |u fzj |
| 245 | _ | _ | |a Structural and transport properties of lithium-conducting NASICON materials |
| 260 | _ | _ | |a New York, NY [u.a.] |c 2018 |b Elsevier |
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| 520 | _ | _ | |a Lithium-containing NASICON-structured materials are a promising class of solid-state Li-ion conductors for application in electrochemical energy storage devices. Amongst the wide variety of possible compositions the highest conductivities are reported for materials according to the formula Li1+xMx(III)M2−x(IV)(PO4)3, in which the substitution of tetravalent with trivalent metal cations leads to incorporation of additional lithium ions and a higher mobility of the charge carriers.For this study, we surveyed more than 300 research articles about Li-NASICON materials. The relations between composition, structure and conductivity are evaluated to give a comprehensive overview of published data on synthesized compositions. A special focus is laid on Li1+xAlxTi2-x (PO4)3 as the single most conductive and investigated material.The collected conductivities show a wide scattering in a range of 10-10 S cm-1 up to 10-3 S cm-1. The highest values are obtained for materials with M(III) to M(IV) cation ratios of x = 0.3–0.4. Further characteristics for high conductivity are evaluated and the rhombohedral structure as well as cation sizes of around 50–60 p.m. are identified as crucial prerequisites, favoring titanium-based compositions. Considering the evaluated data, selected compositions are suggested for further investigation to support future research. |
| 536 | _ | _ | |a 131 - Electrochemical Storage (POF3-131) |0 G:(DE-HGF)POF3-131 |c POF3-131 |f POF III |x 0 |
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| 700 | 1 | _ | |a Tietz, Frank |0 P:(DE-Juel1)129667 |b 1 |u fzj |
| 700 | 1 | _ | |a Grieshammer, Steffen |0 P:(DE-Juel1)167130 |b 2 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.jpowsour.2018.04.059 |g Vol. 391, p. 1 - 9 |0 PERI:(DE-600)1491915-1 |p 1 - 9 |t Journal of power sources |v 391 |y 2018 |x 0378-7753 |
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