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@ARTICLE{Li:858787,
author = {Li, Dan and Vogel, Bärbel and Müller, Rolf and Bian,
Jianchun and Günther, Gebhard and Li, Qian and Zhang,
Jinqiang and Bai, Zhixuan and Vömel, Holger and Riese,
Martin},
title = {{H}igh tropospheric ozone in {L}hasa within the {A}sian
summer monsoon anticyclone in 2013: influence of convective
transport and stratospheric intrusions},
journal = {Atmospheric chemistry and physics},
volume = {18},
number = {24},
issn = {1680-7324},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {FZJ-2018-07627},
pages = {17979 - 17994},
year = {2018},
abstract = {Balloon-borne measurements of ozone in Lhasa (29.66∘ N,
91.14∘ E; 3650 m above sea level) in August 2013 are
investigated using backward trajectory calculations
performed with the Chemical Lagrangian Model of the
Stratosphere (CLaMS). Measurements show three time periods
characterized by high ozone mixing ratios (OMRs) in the
troposphere on 8, 11, and 18–20 August 2013 during the
Asian summer monsoon (ASM) season. Here, we verified two
different sources for the enhanced ozone values in the
troposphere. First, transport of polluted air from the
boundary layer, and second downward transport from the
stratosphere by stratospheric intrusions. Air pollution from
South Asia through convective and long-range transport plays
a key role in enhancing middle tropospheric OMRs up to
$90 \%$ on 8 August and up to $125 \%$ on 11 August 2013
compared to monthly mean ozone of August 2013. Stratospheric
air intruded from the northern high-latitudes to the
southeastern flank of the ASM anticyclone to the troposphere
and is identified as the source of enhanced ozone according
to backward trajectory calculation and satellite
measurements by the Ozone Monitoring Instrument (OMI) and
the Atmospheric Infrared Sounder (AIRS). Air parcels with
high ozone moved from the high-latitude lower stratosphere
to the middle and upper troposphere. These air parcels are
then transported to Lhasa over long distances and enhanced
upper and middle tropospheric ozone over Lhasa during
18–20 August 2013. Our findings demonstrate that the
strong variability of ozone within the ASM anticyclone in
the free troposphere is caused by transport from very
different regions of the atmosphere.},
cin = {IEK-7},
ddc = {550},
cid = {I:(DE-Juel1)IEK-7-20101013},
pnm = {244 - Composition and dynamics of the upper troposphere and
middle atmosphere (POF3-244)},
pid = {G:(DE-HGF)POF3-244},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000453578900005},
doi = {10.5194/acp-18-17979-2018},
url = {https://juser.fz-juelich.de/record/858787},
}