Journal Article FZJ-2019-01062

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High-performance BaZr 0.35 Ti 0.65 O 3 thin film capacitors with ultrahigh energy storage density and excellent thermal stability

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2018
RSC72819 London

Journal of materials chemistry / A Materials for energy and sustainability A 6(26), 12291 - 12297 () [10.1039/C7TA11109F]

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Abstract: The ability to work at ultralow (−90 °C) or ultrahigh (200 °C) temperature with superior energy storage properties is essential for dielectric capacitors to operate in harsh environments. Here, we realized an ultrahigh recoverable energy density (Wrec) (78.7 J cm−3) and efficiency (η) (80.5%) in BaZr0.35Ti0.65O3 film capacitors through enhancing the breakdown electric field strength at room temperature. Moreover, the BaZr0.35Ti0.65O3 film capacitor exhibits great energy storage properties when measured from −150 °C to 200 °C. Wrec and η can reach the value of 41.9 J cm−3 and 66.4% under an electric strength of 4.0 MV cm−1 even at 200 °C, respectively. Especially, the variation of both Wrec and η at 200 °C during 1 × 106 cycles (ferroelectric fatigue tests) is less than 3%. All these reveal that the BZT film capacitor is a commendable material for application in equipment working in harsh environments.

Classification:

Contributing Institute(s):
  1. Physik Nanoskaliger Systeme (ER-C-1)
Research Program(s):
  1. 143 - Controlling Configuration-Based Phenomena (POF3-143) (POF3-143)

Appears in the scientific report 2018
Database coverage:
Medline ; Allianz-Lizenz / DFG ; Clarivate Analytics Master Journal List ; Current Contents - Engineering, Computing and Technology ; Current Contents - Physical, Chemical and Earth Sciences ; IF >= 5 ; JCR ; National-Konsortium ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Web of Science Core Collection
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 Record created 2019-01-31, last modified 2021-01-30


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