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000863369 1001_ $$0P:(DE-Juel1)168592$$aEhteshami, Niloofar$$b0$$ufzj
000863369 245__ $$aAdiponitrile-based electrolytes for high voltage, graphite-based Li-ion battery
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000863369 520__ $$aOperating high voltage lithium-ion batteries (LIB) is still an obstacle due to the limited anodic stability of state-of-the-art alkyl carbonates-based electrolytes which incorporate ethylene carbonate (EC). Thus, we replace here the widely used ethylene carbonate (EC)/dimethyl carbonate (DMC) solvent formulation by adiponitrile (ADN)/DMC (1/1, wt./wt.), to enable room temperature electrolyte formulations with high anodic stabilities. The possibility of operating graphite with 1 M LiDFOB & 1 M LiFSI ADN/DMC (1/1, wt./wt.) without additive is evidenced, with a clear advantage for the LiDFOB electrolyte. The addition of fluoroethylene carbonate (FEC) as a SEI additive results in improved graphite electrode performance in both cases and, less expectedly, in improved anodic stabilities. Cathodes operating above 4.3 V vs Li+/Li have been paired with graphite as well and allowed improved rate capability as compared to graphite half-cells. The safety of the electrolytes versus a charged graphite anode is improved as compared with state-of-the-art, EC-based electrolytes.
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000863369 7001_ $$0P:(DE-HGF)0$$aEguia-Barrio, Aitor$$b1
000863369 7001_ $$00000-0001-8245-5815$$ade Meatza, Iratxe$$b2
000863369 7001_ $$0P:(DE-HGF)0$$aPorcher, Willy$$b3
000863369 7001_ $$0P:(DE-Juel1)166311$$aPaillard, Elie$$b4$$eCorresponding author
000863369 773__ $$0PERI:(DE-600)1491915-1$$a10.1016/j.jpowsour.2018.07.004$$gVol. 397, p. 52 - 58$$p52 - 58$$tJournal of power sources$$v397$$x0378-7753$$y2018
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000863369 8564_ $$uhttps://juser.fz-juelich.de/record/863369/files/2017-11-15_Adiponitrile_EP_NE-for%20repository.pdf$$yPublished on 2018-07-04. Available in OpenAccess from 2020-07-04.
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