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| 001 | 863369 | ||
| 005 | 20240712113109.0 | ||
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| 100 | 1 | _ | |a Ehteshami, Niloofar |0 P:(DE-Juel1)168592 |b 0 |u fzj |
| 245 | _ | _ | |a Adiponitrile-based electrolytes for high voltage, graphite-based Li-ion battery |
| 260 | _ | _ | |a New York, NY [u.a.] |c 2018 |b Elsevier |
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| 520 | _ | _ | |a Operating high voltage lithium-ion batteries (LIB) is still an obstacle due to the limited anodic stability of state-of-the-art alkyl carbonates-based electrolytes which incorporate ethylene carbonate (EC). Thus, we replace here the widely used ethylene carbonate (EC)/dimethyl carbonate (DMC) solvent formulation by adiponitrile (ADN)/DMC (1/1, wt./wt.), to enable room temperature electrolyte formulations with high anodic stabilities. The possibility of operating graphite with 1 M LiDFOB & 1 M LiFSI ADN/DMC (1/1, wt./wt.) without additive is evidenced, with a clear advantage for the LiDFOB electrolyte. The addition of fluoroethylene carbonate (FEC) as a SEI additive results in improved graphite electrode performance in both cases and, less expectedly, in improved anodic stabilities. Cathodes operating above 4.3 V vs Li+/Li have been paired with graphite as well and allowed improved rate capability as compared to graphite half-cells. The safety of the electrolytes versus a charged graphite anode is improved as compared with state-of-the-art, EC-based electrolytes. |
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| 700 | 1 | _ | |a Eguia-Barrio, Aitor |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a de Meatza, Iratxe |0 0000-0001-8245-5815 |b 2 |
| 700 | 1 | _ | |a Porcher, Willy |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Paillard, Elie |0 P:(DE-Juel1)166311 |b 4 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.jpowsour.2018.07.004 |g Vol. 397, p. 52 - 58 |0 PERI:(DE-600)1491915-1 |p 52 - 58 |t Journal of power sources |v 397 |y 2018 |x 0378-7753 |
| 856 | 4 | _ | |y Restricted |u https://juser.fz-juelich.de/record/863369/files/1-s2.0-S0378775318307134-main.pdf |
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| 856 | 4 | _ | |y Published on 2018-07-04. Available in OpenAccess from 2020-07-04. |u https://juser.fz-juelich.de/record/863369/files/2017-11-15_Adiponitrile_EP_NE-for%20repository.pdf |
| 856 | 4 | _ | |y Published on 2018-07-04. Available in OpenAccess from 2020-07-04. |x pdfa |u https://juser.fz-juelich.de/record/863369/files/2017-11-15_Adiponitrile_EP_NE-for%20repository.pdf?subformat=pdfa |
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