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@ARTICLE{Mechsner:864465,
      author       = {Mechsner, Bastian and Böse, Dietrich and Hogenkamp, Fabian
                      and Ledermann, Nadia and Hartmann, Rudolf and Bochinsky,
                      Kevin and Frey, Wolfgang and Pietruszka, Jörg},
      title        = {{E}nantioselective total synthesis of altersolanol {A} and
                      {N}},
      journal      = {Bioorganic $\&$ medicinal chemistry},
      volume       = {27},
      number       = {13},
      issn         = {0968-0896},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2019-04246},
      pages        = {2991 - 2997},
      year         = {2019},
      abstract     = {The development of the first enantioselective total
                      synthesis of altersolanol N is reported. The decisive step
                      of the synthesis is the enantioselective formation of the
                      tetrahydroanthraquinone nucleus by a
                      [4 + 2]-cycloaddition in high yield and with excellent
                      diastereo- and enantioselectivity (>95:5 dr and 95:5 er). In
                      addition, a demanding selective monoacetylation of the OH
                      group at the C-2 position was achieved: an epoxide ring
                      opening with the participation of a neighbouring acetyl
                      group could be established. The route proved to be an
                      efficient alternative to also access enantiomerically pure
                      altersolanol A.},
      cin          = {IBOC / IBG-1 / ICS-6},
      ddc          = {610},
      cid          = {I:(DE-Juel1)IBOC-20090406 / I:(DE-Juel1)IBG-1-20101118 /
                      I:(DE-Juel1)ICS-6-20110106},
      pnm          = {581 - Biotechnology (POF3-581)},
      pid          = {G:(DE-HGF)POF3-581},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:31072649},
      UT           = {WOS:000470106900027},
      doi          = {10.1016/j.bmc.2019.04.033},
      url          = {https://juser.fz-juelich.de/record/864465},
}