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100 1 _ |a Mei, Antonio B.
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245 _ _ |a Self-assembly and properties of domain walls in BiFeO3 layers grown via molecular-beam epitaxy
260 _ _ |a Melville, NY
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520 _ _ |a Bismuth ferrite layers, ∼200-nm-thick, are deposited on SrRuO 3 -coated DyScO 3 (110) o substrates in a step-flow growth regime via adsorption-controlled molecular-beam epitaxy. Structural characterization shows the films to be phase pure with substrate-limited mosaicity (0.012 ○x-ray diffraction ω-rocking curve widths). The film surfaces are atomically smooth (0.2 nm root-mean-square height fluctuations) and consistof 260-nm-wide [11̄1] o -oriented terraces and unit-cell-tall (0.4 nm) step edges. The combination of electrostatic and symmetry boundaryconditions promotes two monoclinically distorted BiFeO 3 ferroelectric variants, which self-assemble into a pattern with unprecedentedlycoherent periodicity, consisting of 145 ± 2-nm-wide stripe domains separated by [001] o -oriented 71 ○ domain walls. The walls exhibit electricalrectification and enhanced conductivity.
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700 1 _ |a Tang, Yongjian
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700 1 _ |a Jena, Debdeep
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700 1 _ |a Schlom, Darrell G.
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773 _ _ |a 10.1063/1.5103244
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