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@ARTICLE{Zhang:865751,
author = {Zhang, Shidong and Beale, Steven and Reimer, Uwe and
Andersson, Martin and Lehnert, Werner},
title = {{P}olymer electrolyte fuel {C}ell {M}odeling - {C}omparison
of {T}wo {M}odels with {D}ifferent {L}evels of {C}omplexity},
journal = {International journal of hydrogen energy},
volume = {45},
number = {38},
issn = {0360-3199},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2019-05067},
pages = {19761 - 19777},
year = {2020},
abstract = {The modeling of fuel cells requires the coupling of fluid
transport with electro-chemical reactions. There are two
approaches commonly used. Firstly, the electrodes can be
treated as two planes, where the potential gradient can be
considered as being locally one-dimensional. In this case a
two dimensional current density distribution is obtained.
Secondly, the two electrode layers can be spatially resolved
and the protonic and electronic potentials obtained by
solving a pair of coupled Poisson equations. The latter
approach requires much higher computational resources,
because a higher spatial resolution is required and a large
set of model parameters is required. On the other hand, much
more detailed local information can be obtained by this
method. The motivation for this study was to compare the
results quantitively with detailed experimental data for a
high temperature polymer electrolyte fuel cell with a
geometric area of 200 cm2. Both model approaches show very
good agreement with measured local current density
distributions. The second model is able to provide a deeper
insight into the current density variation through the
membrane and catalyst layers and reveals points with local
extremes. The present results are specific for high
temperature polymer electrolyte fuel cells but the
conclusions may readily be applied to the modeling of other
high temperature fuel cell types.},
cin = {IEK-14},
ddc = {620},
cid = {I:(DE-Juel1)IEK-14-20191129},
pnm = {135 - Fuel Cells (POF3-135)},
pid = {G:(DE-HGF)POF3-135},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000552053500085},
doi = {10.1016/j.ijhydene.2020.05.060},
url = {https://juser.fz-juelich.de/record/865751},
}