TY - JOUR
AU - Lee, S. W.
AU - Guo, H.
AU - Zhao, L.
AU - Hu, Z.
AU - Müller, Thomas
AU - Lin, H. J.
AU - Chen, C. T.
AU - Ryu, G.
AU - Tjeng, L. H.
AU - Komarek, A. C.
TI - Cu2MSiO5 (M = Co , Ni) : A new silicate material with chains of Cu and M ions
JO - Physical review materials
VL - 3
IS - 3
SN - 2475-9953
CY - College Park, MD
PB - APS
M1 - FZJ-2019-05505
SP - 034408
PY - 2019
AB - We report on the synthesis of a new material with a novel quasi-one-dimensional crystal structure consisting of chains of Cu and M ions: Cu2MSiO5 with M = Co, Ni. Large, centimeter-sized single crystals of Cu2CoSiO5 have been grown by the floating-zone technique and roughly hexagonally shaped single crystals of Cu2NiSiO5 have been grown by means of chemical vapor transport. Cu2CoSiO5 (Cu2NiSiO5) orders antiferromagnetically below TN∼ 15 K (12.5 K). Polarized neutron scattering experiments on Cu2CoSiO5 reveal incommensurate magnetism below TN with propagation vectors k±=±(∼0.200.3), and magnetic susceptibility measurements indicate a large unquenched orbital moment of about 1μB per Co ion.
LB - PUB:(DE-HGF)16
UR - <Go to ISI:>//WOS:000461938500002
DO - DOI:10.1103/PhysRevMaterials.3.034408
UR - https://juser.fz-juelich.de/record/866349
ER -