Journal Article

FZJ-2019-05588

http://join2-wiki.gsi.de/foswiki/pub/Main/Artwork/join2_logo100x88.png Three-dimensional tomographic imaging of molecular orbitals by photoelectron momentum microscopy

Graus, M. ; Metzger, C. ; Grimm, M. ; Nigge, P. ; Feyer, V.FZJ* ; Schöll, A. (Corresponding author) ; Reinert, F.

2019
Springer Heidelberg

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Please use a persistent id in citations: doi:10.1140/epjb/e2019-100015-x

Abstract: As one of the fundamental concepts of quantum mechanics, electrons in atoms and molecules are assigned to respective orbitals. The geometric distribution of these orbitals is immediately connected to many chemical and physical properties of the system. Consequently, measuring electron orbitals directly has been highly desired. In this study, we demonstrate how a combination of a photoemission electron microscope with a synchrotron UV-light source can be utilised to record a three-dimensional set of tomographic data and present a detailed procedure to reconstruct the orbitals under investigation in real space.

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Contributing Institute(s):

1. Elektronische Eigenschaften (PGI-6)

Research Program(s):

1. 522 - Controlling Spin-Based Phenomena (POF3-522) (POF3-522)

Appears in the scientific report 2019

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Database coverage:
; Clarivate Analytics Master Journal List ; Current Contents - Physical, Chemical and Earth Sciences ; Ebsco Academic Search ; IF < 5 ; JCR ; Nationallizenz ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Web of Science Core Collection

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