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@ARTICLE{Kim:867277,
      author       = {Kim, Un-Hyuck and Kuo, Liang-Yin and Kaghazchi, Payam and
                      Yoon, Chong S. and Sun, Yang-Kook},
      title        = {{Q}uaternary {L}ayered {N}i-{R}ich {NCMA} {C}athode for
                      {L}ithium-{I}on {B}atteries},
      journal      = {ACS energy letters},
      volume       = {4},
      number       = {2},
      issn         = {2380-8195},
      address      = {Washington, DC},
      publisher    = {American Chemical Society},
      reportid     = {FZJ-2019-06035},
      pages        = {576 - 582},
      year         = {2019},
      abstract     = {Li[Ni1–x–yCoxAly]O2 (NCA) and Li[Ni1–x–yCoxMny]O2
                      (NCM) cathodes have been the archetypes of current
                      high-energy-density cathodes for Li-ion batteries. A hybrid
                      of NCA and NCM cathodes, a quaternary system consisting of
                      Li[Ni0.89Co0.05Mn0.05Al0.01]O2 (NCMA) was benchmarked
                      against NCM and NCA with similar Ni contents. The quaternary
                      NCMA cathode delivered a capacity of 228 mAh g–1 and
                      outperformed the benchmarking cathodes in long-term cycling
                      stability $(85\%$ after 1000 cycles). The reduction in the
                      volume change during deintercalation and the enhanced
                      intrinsic mechanical strength confirmed by the
                      single-particle compression test suppressed the microcrack
                      nucleation and propagation. Microcrack suppression was
                      important because microcracks serve as channels for
                      electrolyte infiltration and lead to subsequent surface
                      degradation of internal surfaces. The proposed NCMA cathode
                      provides extra cycling stability, which is essential for
                      electric vehicles, which require a long battery life and
                      improves the thermal stability of the cathode, which
                      contributes to a safer battery.},
      cin          = {IEK-1},
      ddc          = {333.7},
      cid          = {I:(DE-Juel1)IEK-1-20101013},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000458938400030},
      doi          = {10.1021/acsenergylett.8b02499},
      url          = {https://juser.fz-juelich.de/record/867277},
}