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@ARTICLE{Mishra:873679,
author = {Mishra, Tarini Prasad and Neto, Rubens Roberto Ingraci and
Speranza, Giorgio and Quaranta, Alberto and Sglavo, Vincenzo
M. and Raj, Rishi and Guillon, Olivier and Bram, Martin and
Biesuz, Mattia},
title = {{E}lectronic conductivity in gadolinium doped ceria under
direct current as a trigger for flash sintering},
journal = {Scripta materialia},
volume = {179},
issn = {1359-6462},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2020-00908},
pages = {55 - 60},
year = {2020},
abstract = {In this paper, we discuss the progression of flash
sintering in $10mol\%$ gadolinium-doped ceria specimens.
Flash transition is correlated with the generation of n-type
electronic conductivity in air under direct-current bias.
Its origin is attributed to partial reduction of the
material which propagates from the cathodic-to-anodic
region. The phenomenon was observed, in-situ, by monitoring
the development of electrochemical blackening during the
incubation period of the flash-experiment. Anomalous
features, including shift in the valence band edge,
shrinkage of the band-gap and change in the oxidation state
of Ce in flashed samples was confirmed by X-ray
photoelectron spectroscopy and diffuse reflectance
measurements.},
cin = {IEK-1},
ddc = {670},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {899 - ohne Topic (POF3-899) / DFG project 274005202 - SPP
1959: Manipulation of matter controlled by electric and
magnetic fields: Towards novel synthesis and processing
routes of inorganic materials (274005202)},
pid = {G:(DE-HGF)POF3-899 / G:(GEPRIS)274005202},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000514758200012},
doi = {10.1016/j.scriptamat.2020.01.007},
url = {https://juser.fz-juelich.de/record/873679},
}