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@ARTICLE{Herrmann:875055,
author = {Herrmann, Markus and Stoffel, Ralf P. and Sergueev, Ilya
and Wille, Hans-Christian and Leupold, Olaf and Ait
Haddouch, Mohammed and Sala, Gabriele and Abernathy, Doug L.
and Voigt, Jörg and Hermann, Raphaël P. and Dronskowski,
Richard and Friese, Karen},
title = {{L}attice {D}ynamics of {S}b 2 {S}e 3 from {I}nelastic
{N}eutron and {X}‐{R}ay {S}cattering},
journal = {Physica status solidi / B Basic research B},
volume = {257},
number = {6},
issn = {1521-3951},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2020-01776},
pages = {2000063},
year = {2020},
abstract = {The lattice dynamics of orthorhombic Sb2Se3 is studied by a
combination of inelastic neutron and 121Sb nuclear inelastic
scattering giving access to the total and Sb partial density
of phonon states (DPS). The Se partial DPS is determined
from the difference between the total and Sb partial DPS.
The total DPS is determined at 39, 150, and 300 K, and an
analysis of the temperature‐induced mode shifts in
combination with low‐temperature powder diffraction data
is provided. Using an earlier reported theoretical approach,
the corresponding total and partial DPS of Sb2Se3 are
calculated by first‐principles calculations. Herein, a
detailed analysis of the Grüneisen parameter,
element‐specific and bulk Debye temperatures, and the mean
force constants as derived from the experimental data and
discrete Fourier transform calculations is provided. In
general, the calculations underestimate the strength of the
covalent SbSe bonds.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / JARA-HPC},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6212 - Quantum
Condensed Matter: Magnetism, Superconductivity (POF3-621) /
6213 - Materials and Processes for Energy and Transport
Technologies (POF3-621) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (POF3-623) / Quantum chemistry of functional
chalcogenide for phase-change memories and other
applications $(jara0033_20171101)$},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-6213 /
G:(DE-HGF)POF3-6G4 / $G:(DE-Juel1)jara0033_20171101$},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000527883000001},
doi = {10.1002/pssb.202000063},
url = {https://juser.fz-juelich.de/record/875055},
}