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000875172 1001_ $$0P:(DE-Juel1)173726$$aTan, Zhaofeng$$b0$$ufzj
000875172 245__ $$aNo Evidence for a Significant Impact of Heterogeneous Chemistry on Radical Concentrations in the North China Plain in Summer 2014
000875172 260__ $$aColumbus, Ohio$$bAmerican Chemical Society$$c2020
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000875172 520__ $$aThe oxidation of nitric oxide to nitrogen dioxide by hydroperoxy (HO2) and organic peroxy radicals (RO2) is responsible for the chemical net ozone production in the troposphere and for the regeneration of hydroxyl radicals, the most important oxidant in the atmosphere. In Summer 2014, a field campaign was conducted in the North China Plain, where increasingly severe ozone pollution has been experienced in the last years. Chemical conditions in the campaign were representative for this area. Radical and trace gas concentrations were measured, allowing for calculating the turnover rates of gas-phase radical reactions. Therefore, the importance of heterogeneous HO2 uptake on aerosol could be experimentally determined. HO2 uptake could have suppressed ozone formation at that time because of the competition with gas-phase reactions that produce ozone. The successful reduction of the aerosol load in the North China Plain in the last years could have led to a significant decrease of HO2 loss on particles, so that ozone-forming reactions could have gained importance in the last years. However, the analysis of the measured radical budget in this campaign shows that HO2 aerosol uptake did not impact radical chemistry for chemical conditions in 2014. Therefore, reduced HO2 uptake on aerosol since then is likely not the reason for the increasing number of ozone pollution events in the North China Plain, contradicting conclusions made from model calculations reported in the literature.
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000875172 7001_ $$0P:(DE-Juel1)16326$$aHofzumahaus, Andreas$$b1$$ufzj
000875172 7001_ $$0P:(DE-Juel1)6776$$aLu, Keding$$b2
000875172 7001_ $$0P:(DE-HGF)0$$aBrown, Steven S.$$b3
000875172 7001_ $$0P:(DE-Juel1)16342$$aHolland, Frank$$b4$$ufzj
000875172 7001_ $$0P:(DE-HGF)0$$aHuey, Lewis Gregory$$b5
000875172 7001_ $$0P:(DE-Juel1)4528$$aKiendler-Scharr, Astrid$$b6$$ufzj
000875172 7001_ $$0P:(DE-HGF)0$$aLi, Xin$$b7
000875172 7001_ $$0P:(DE-HGF)0$$aLiu, Xiaoxi$$b8
000875172 7001_ $$0P:(DE-HGF)0$$aMa, Nan$$b9
000875172 7001_ $$0P:(DE-HGF)0$$aMin, Kyung-Eun$$b10
000875172 7001_ $$0P:(DE-Juel1)16347$$aRohrer, Franz$$b11$$ufzj
000875172 7001_ $$0P:(DE-HGF)0$$aShao, Min$$b12
000875172 7001_ $$0P:(DE-Juel1)16324$$aWahner, Andreas$$b13$$ufzj
000875172 7001_ $$0P:(DE-HGF)0$$aWang, Yuhang$$b14
000875172 7001_ $$0P:(DE-HGF)0$$aWiedensohler, Alfred$$b15
000875172 7001_ $$0P:(DE-HGF)0$$aWu, Yusheng$$b16
000875172 7001_ $$0P:(DE-HGF)0$$aWu, Zhijun$$b17
000875172 7001_ $$0P:(DE-HGF)0$$aZeng, Limin$$b18
000875172 7001_ $$0P:(DE-HGF)0$$aZhang, Yuanhang$$b19
000875172 7001_ $$0P:(DE-Juel1)7363$$aFuchs, Hendrik$$b20$$eCorresponding author
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