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@ARTICLE{Yao:875205,
author = {Yao, Zhirong and Cai, Lun and Meng, Lanxiang and Qiu, Kaifu
and Lin, Wenjie and Jin, Jingsheng and Duan, Weiyuan and
Ding, Kaining and Li, Shenghao and Ai, Bin and Liang,
Zongcun and Shen, Hui},
title = {{H}igh‐{P}erformance and {S}table {D}opant‐{F}ree
{S}ilicon {S}olar {C}ells with {M}agnesium {A}cetylacetonate
{E}lectron‐{S}elective {C}ontacts},
journal = {Physica status solidi / Rapid research letters Rapid
research letters},
volume = {14},
number = {6},
issn = {1862-6270},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2020-01873},
pages = {2000103},
year = {2020},
abstract = {One of the challenges in fabricating high‐performance
n‐type crystalline silicon (n‐type c‐Si) solar cells
is the high‐quality n‐type c‐Si/metal contact.
Schottky barriers are commonly found on the n‐type
c‐Si/metal contact, which suppresses electron
transportation. Herein, novel stacks of magnesium
acetylacetonate (Mg(Acac)2)/magnesium (Mg)/silver (Ag) to
form electron‐selective contacts for n‐type c‐Si solar
cells are presented, which enables a dopant‐free process.
An ohmic contact on n‐type c‐Si is formed using the
Mg(Acac)2/Mg/Ag stacks. The transmission spectrum and
ultraviolet photoelectron spectroscopy measurements show
negligible conduction‐band offset and large valence‐band
offset between Mg(Acac)2 and n‐type c‐Si, which
indicates the electron‐transporting and hole‐blocking
properties of Mg(Acac)2/n‐type c‐Si heterocontacts.
Moreover, the contact resistivities (ρ c ) between the
Mg(Acac)2/Mg/Ag electron‐selective heterocontacts and
n‐type c‐Si substrates are lower than 10 mΩ cm2,
which demonstrates the good electrode properties of the
Mg(Acac)2/Mg/Ag stacks. The Mg(Acac)2/Mg/Ag
electron‐selective stacks are applied on n‐type c‐Si
solar cells with partial rear contact, and $>20\%$
efficiency is achieved, which is higher than that in a
reference cell with only Ag contact. The stability of the
n‐type c‐Si solar cell performance equipped with
Mg(Acac)2/Mg/Ag contacts is verified under ambient
conditions. This novel low‐temperature contact technique
offers a reliable alternative for high‐performance
n‐type c‐Si solar cells.},
cin = {IEK-5},
ddc = {530},
cid = {I:(DE-Juel1)IEK-5-20101013},
pnm = {121 - Solar cells of the next generation (POF3-121)},
pid = {G:(DE-HGF)POF3-121},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000528615100001},
doi = {10.1002/pssr.202000103},
url = {https://juser.fz-juelich.de/record/875205},
}