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@ARTICLE{Kretzschmar:875336,
      author       = {Kretzschmar, Ansgar and Selmert, Victor and Weinrich,
                      Henning and Kungl, Hans and Tempel, Hermann and Eichel,
                      Rüdiger‐A.},
      title        = {{T}ailored {G}as {A}dsorption {P}roperties of {E}lectrospun
                      {C}arbon {N}anofibers for {G}as {S}eparation and {S}torage},
      journal      = {ChemSusChem},
      volume       = {13},
      number       = {12},
      issn         = {1864-564X},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2020-01959},
      pages        = {3180-3191},
      year         = {2020},
      abstract     = {Carbon nanofibers (CNFs) derived from electrospun
                      polyacrylonitrile (PAN) were investigated with respect to
                      their gas adsorption properties. By employing CO2 adsorption
                      measurements, it is shown that the adsorption capacity and
                      selectivity of the fibers can be tailored by means of the
                      applied carbonization temperature. General pore properties
                      of the CNFs were identified by Ar adsorption measurements,
                      whereas CO2 adsorption measurements provided information
                      about the ultramicroporosity, adsorption energies, and
                      adsorption capacities. Ideal adsorbed solution theory (IAST)
                      selectivities under practically relevant conditions were
                      determined by evaluation of single‐component data for N2
                      and CO2. Especially for low carbonization temperatures, the
                      CNFs exhibit very good low‐pressure adsorption performance
                      and excellent CO2/N2 IAST selectivities of 350 at 20 mbar
                      and 132 at 1 bar, which are attributed to a
                      molecular‐sieve effect in very narrow slit pores. These
                      IAST selectivities are some of the highest values for carbon
                      materials reported in the literature so far and the highest
                      IAST selectivities for as‐prepared, non‐post‐treated
                      carbon ever.},
      cin          = {IEK-9},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {131 - Electrochemical Storage (POF3-131) / HITEC -
                      Helmholtz Interdisciplinary Doctoral Training in Energy and
                      Climate Research (HITEC) (HITEC-20170406)},
      pid          = {G:(DE-HGF)POF3-131 / G:(DE-Juel1)HITEC-20170406},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:32216123},
      UT           = {WOS:000530075600001},
      doi          = {10.1002/cssc.202000520},
      url          = {https://juser.fz-juelich.de/record/875336},
}