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@ARTICLE{Basak:875392,
      author       = {Basak, Shibabrata and Migunov, Vadim and Tavabi, Amir
                      Hossein and George, Chandramohan and Lee, Qing and Rosi,
                      Paolo and Arszelewska, Violetta and Ganapathy, Swapna and
                      Vijay, Ashwin and Ooms, Frans G. B. and Schierholz, Roland
                      and Tempel, Hermann and Kungl, Hans and Mayer, Joachim and
                      Dunin-Borkowski, Rafal E. and Eichel, Rüdiger-A. and
                      Wagemaker, Marnix and Kelder, Erik M.},
      title        = {{O}perando {T}ransmission {E}lectron {M}icroscopy {S}tudy
                      of {A}ll-{S}olid-{S}tate {B}attery {I}nterface:
                      {R}edistribution of {L}ithium among {I}nterconnected
                      {P}articles},
      journal      = {ACS applied energy materials},
      volume       = {3},
      number       = {6},
      issn         = {2574-0962},
      address      = {Washington, DC},
      publisher    = {ACS Publications},
      reportid     = {FZJ-2020-02001},
      pages        = {5101–5106},
      year         = {2020},
      note         = {Grant: BMBF projects−CatSE (Project 13XP0223A) and LiSi
                      (Project 13XP0224B)},
      abstract     = {With operando transmission electron microscopy visualizing
                      solid-solid electrode-electrolyte interface of silicon
                      active particles and lithium oxide solid electrolyte as a
                      model system, we show that (de)lithiation (battery cycling)
                      does not require all particles to be in direct contact with
                      electrolytes across length scales of few hundreds of
                      nanometer. A facile lithium redistribution that occurs
                      between interconnected active particles indicates that
                      lithium does not necessarily become isolated in individual
                      particles due to loss of a direct contact. Our results have
                      implications for the design of all-solid-state battery
                      electrodes with improved capacity retention and
                      cyclability.},
      cin          = {IEK-9 / ER-C-1 / ER-C-2},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-9-20110218 / I:(DE-Juel1)ER-C-1-20170209 /
                      I:(DE-Juel1)ER-C-2-20170209},
      pnm          = {131 - Electrochemical Storage (POF3-131) / 143 -
                      Controlling Configuration-Based Phenomena (POF3-143) / DFG
                      project 167917811 - SFB 917: Resistiv schaltende
                      Chalkogenide für zukünftige Elektronikanwendungen:
                      Struktur, Kinetik und Bauelementskalierung "Nanoswitches"
                      (167917811)},
      pid          = {G:(DE-HGF)POF3-131 / G:(DE-HGF)POF3-143 /
                      G:(GEPRIS)167917811},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000543715100002},
      doi          = {10.1021/acsaem.0c00543},
      url          = {https://juser.fz-juelich.de/record/875392},
}