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100 1 _ |a Basak, Shibabrata
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245 _ _ |a Operando Transmission Electron Microscopy Study of All-Solid-State Battery Interface: Redistribution of Lithium among Interconnected Particles
260 _ _ |a Washington, DC
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500 _ _ |a Grant: BMBF projects−CatSE (Project 13XP0223A) and LiSi (Project 13XP0224B)
520 _ _ |a With operando transmission electron microscopy visualizing solid-solid electrode-electrolyte interface of silicon active particles and lithium oxide solid electrolyte as a model system, we show that (de)lithiation (battery cycling) does not require all particles to be in direct contact with electrolytes across length scales of few hundreds of nanometer. A facile lithium redistribution that occurs between interconnected active particles indicates that lithium does not necessarily become isolated in individual particles due to loss of a direct contact. Our results have implications for the design of all-solid-state battery electrodes with improved capacity retention and cyclability.
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773 _ _ |a 10.1021/acsaem.0c00543
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