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@ARTICLE{Qdemat:877585,
author = {Qdemat, Asma and Kentzinger, Emmanuel and Buitenhuis, Johan
and Rücker, Ulrich and Ganeva, Marina and Brückel, Thomas},
title = {{S}elf assembled monolayer of silica nanoparticles with
improved order by drop casting},
journal = {RSC Advances},
volume = {10},
number = {31},
issn = {2046-2069},
address = {London},
publisher = {RSC Publishing},
reportid = {FZJ-2020-02307},
pages = {18339 - 18347},
year = {2020},
abstract = {This paper reports on the formation of large area, self
assembled, highly ordered monolayers of stearyl alcohol
grafted silica nanospheres of ≈50 nm diameter on a silicon
substrate based on the drop-casting method. Our novel
approach to achieve improved order uses stearyl alcohol as
an assistant by adding it to the colloidal NanoParticle (NP)
dispersion from which the monolayers are formed.
Additionally, a heat treatment step is added, to melt the
stearyl alcohol in the monolayer and thereby give the
particles more time to further self-assemble, leading to
additional improvement in the monolayer quality. The
formation of the monolayers is significantly affected by the
concentration of the NPs and the stearyl alcohol, the volume
of the drop as well as the time of the heat treatment. A
high surface coverage and uniform monolayer film of SiO2 NPs
is achieved by appropriate control of the above-mentioned
preparation parameters. Structural characterization of the
obtained SiO2 NP monolayer was done locally by Scanning
Electron Microscopy (SEM), and globally by X-ray
reflectivity (XRR) and grazing incidence small-angle X-ray
scattering (GISAXS), where the data was reproduced by
simulation within the Distorted Wave Born Approximation
(DWBA). In conclusion, our modified drop-casting method is a
simple, inexpensive method, which provides highly ordered
self-assembled monolayers of silica particles, if combined
with a compatible additive and a heat treatment step. This
method might be more general and also applicable to
different particles after finding an appropriate additive.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / IBI-4 / JCNS-HBS / JCNS-FRM-II},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ / I:(DE-Juel1)IBI-4-20200312 /
I:(DE-Juel1)JCNS-HBS-20180709 /
I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6212 - Quantum
Condensed Matter: Magnetism, Superconductivity (POF3-621) /
6213 - Materials and Processes for Energy and Transport
Technologies (POF3-621) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-6213 /
G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000537264400041},
doi = {10.1039/D0RA00936A},
url = {https://juser.fz-juelich.de/record/877585},
}