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@ARTICLE{Chiesa:885419,
author = {Chiesa, A. and Macaluso, E. and Santini, P. and Carretta,
S. and Pavarini, E.},
title = {{F}irst-principles many-body models for electron transport
through molecular nanomagnets},
journal = {Physical review / B},
volume = {99},
number = {23},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2020-03816},
pages = {235145},
year = {2019},
abstract = {Impressive advances in the field of molecular spintronics
allow one to study electron transport through individual
magnetic molecules embedded between metallic leads in the
purely quantum regime of single electron tunneling. Besides
fundamental interest, this experimental setup, in which a
single molecule is manipulated by electronic means, provides
the elementary units of possible forthcoming technological
applications, ranging from spin valves to transistors and
qubits for quantum information processing. Theoretically,
while for weakly correlated molecular junctions established
first-principles techniques do enable the system-specific
description of transport phenomena, methods of similar power
and flexibility are still lacking for junctions involving
strongly correlated molecular nanomagnets. Here we propose
an efficient scheme based on the ab initio construction of
material-specific Hubbard models and on the master-equation
formalism. We apply this approach to a representative case,
the {$Ni_2$} molecular spin dimer, in the regime of weak
molecule-electrode coupling, the one relevant for
quantum-information applications. Our approach allows us to
study in a realistic setting many-body effects such as
current suppression and negative differential conductance.
We think that this method has the potential for becoming a
very useful tool for describing transport phenomena in
strongly correlated molecules.},
ddc = {530},
pnm = {Spin-orbital order-disorder transitions in strongly
correlated systems $(jiff46_20161101)$},
pid = {$G:(DE-Juel1)jiff46_20161101$},
typ = {PUB:(DE-HGF)16},
doi = {10.1103/PhysRevB.99.235145},
url = {https://juser.fz-juelich.de/record/885419},
}