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000890727 1001_ $$0P:(DE-Juel1)173073$$aKrückemeier, Lisa$$b0$$eCorresponding author$$ufzj
000890727 245__ $$aUnderstanding Transient Photoluminescence in Halide Perovskite Layer Stacks and Solar Cells
000890727 260__ $$aWeinheim$$bWiley-VCH$$c2021
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000890727 520__ $$aWhile transient photoluminescence (TPL) measurements are a very popular tool to monitor the charge-carrier dynamics in the field of halide perovskite photovoltaics, interpretation of data obtained on multilayer samples is highly challenging due to the superposition of various effects that modulate the charge-carrier concentration in the perovskite layer and thereby the measured photoluminescence (PL). These effects include bulk and interfacial recombination, charge transfer to electron- or hole transport layers, and capacitive charging or discharging. Here, numerical simulations with Sentauraus TCAD, analytical solutions, and experimental data with a dynamic range of ≈7 orders of magnitude on a variety of different sample geometries, from perovskite films on glass to full devices, are combined to present an improved understanding of this method. A presentation of the decay time of the TPL decay that follows from taking the derivative of the photoluminescence at every time is proposed. Plotting this decay time as a function of the time-dependent quasi-Fermi-level splitting enables distinguishing between the different contributions of radiative and non-radiative recombination as well as charge extraction and capacitive effects to the decay.
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000890727 7001_ $$0P:(DE-Juel1)169731$$aKrogmeier, Benedikt$$b1$$ufzj
000890727 7001_ $$0P:(DE-Juel1)169264$$aLiu, Zhifa$$b2$$ufzj
000890727 7001_ $$0P:(DE-Juel1)143905$$aRau, Uwe$$b3$$ufzj
000890727 7001_ $$0P:(DE-Juel1)159457$$aKirchartz, Thomas$$b4$$eCorresponding author
000890727 773__ $$0PERI:(DE-600)2594556-7$$a10.1002/aenm.202003489$$n19$$p202003489$$tAdvanced energy materials$$v11$$x1614-6832$$y2021
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