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@ARTICLE{Chen:890728,
      author       = {Chen, Chunguang and Jiang, Ming and Zhou, Tao and
                      Raijmakers, Luc and Vezhlev, Egor and Wu, Baolin and
                      Schülli, Tobias U. and Danilov, Dmitri L. and Wei, Yujie
                      and Eichel, Rüdiger-A. and Notten, Peter H. L.},
      title        = {{I}nterface {A}spects in {A}ll‐{S}olid‐{S}tate
                      {L}i‐{B}ased {B}atteries {R}eviewed},
      journal      = {Advanced energy materials},
      volume       = {11},
      number       = {13},
      issn         = {1614-6840},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2021-01151},
      pages        = {2003939 -},
      year         = {2021},
      abstract     = {Extensive efforts have been made to improve the Li-ionic
                      conductivity of solid electrolytes (SE) for developing
                      promising all-solid-state Li-based batteries (ASSB). Recent
                      studies suggest that minimizing the existing interface
                      problems is even more important than maximizing the
                      conductivity of SE. Interfaces are essential in ASSB, and
                      their properties significantly influence the battery
                      performance. Interface problems, arising from both physical
                      and (electro)chemical material properties, can significantly
                      inhibit the transport of electrons and Li-ions in ASSB.
                      Consequently, interface problems may result in interlayer
                      formation, high impedances, immobilization of moveable
                      Li-ions, loss of active host sites available to accommodate
                      Li-ions, and Li-dendrite formation, all causing significant
                      storage capacity losses and ultimately battery failures. The
                      characteristic differences of interfaces between liquid- and
                      solid-type Li-based batteries are presented here. Interface
                      types, interlayer origin, physical and chemical structures,
                      properties, time evolution, complex interrelations between
                      various factors, and promising interfacial tailoring
                      approaches are reviewed. Furthermore, recent advances in the
                      interface-sensitive or depth-resolved analytical tools that
                      can provide mechanistic insights into the interlayer
                      formation and strategies to tailor the interlayer formation,
                      composition, and properties are discussed.},
      cin          = {IEK-9},
      ddc          = {050},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {123 - Chemische Energieträger (POF4-123)},
      pid          = {G:(DE-HGF)POF4-123},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000618968600001},
      doi          = {10.1002/aenm.202003939},
      url          = {https://juser.fz-juelich.de/record/890728},
}