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| 100 | 1 | _ | |a Korshunov, Aleksandr |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Host‐Guest Interactions Enhance the Performance of Viologen Electrolytes for Aqueous Organic Redox Flow Batteries |
| 260 | _ | _ | |a Weinheim |c 2021 |b Wiley-VCH |
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| 520 | _ | _ | |a Host-guest interactions are an attractive approach to design redox electrolytes, enabling to precisely tune the key properties for redox flow batteries such as half-cell redox potential, solubility, and stability. Herein we report a host-guest complex of highly water soluble (2-hydroxypropyl)-β-cyclodextrin with 1-decyl-1′-ethyl-4,4′-bipyridinium dibromide as anolyte in a new aqueous organic redox flow battery (AORFB). The supramolecular anolyte ensured the total RFB voltage increase of ≈9 % up to 0.97 V and provided a stable capacity delivery for more than 500 cycles with a capacity fade rate of 0.037 %/cycle (2.84 %/day) at high Coulombic (>99.5 %) and energy (>62 %) efficiencies. The results highlight host-guest interactions as promising strategy towards more effective storage of renewable energy within AORFBs. |
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