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@ARTICLE{Mi:892556,
author = {Mi, Xinrun and Wang, Xiao and Gui, Hengrui and Pi, Maocai
and Zheng, Tingting and Yang, Kunya and Gan, Yuhan and Wang,
Peipei and Li, Alei and Wang, Aifeng and Zhang, Liyuan and
Su, Yixi and Chai, Yisheng and He, Mingquan},
title = {{S}tacking faults in α−{R}u{C}l3 revealed by local
electric polarization},
journal = {Physical review / B},
volume = {103},
number = {17},
issn = {2469-9969},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2021-02155},
pages = {174413},
year = {2021},
abstract = {We present out-of-plane dielectric and magnetodielectric
measurements of single-crystalline α−RuCl3 with various
degrees of stacking faults. A frequency-dependent, but
field-independent, dielectric anomaly appears at
TA(f=100kHz)∼4 K once both magnetic transitions at TN1∼7
K and TN2∼14 K set in. The observed dielectric anomaly is
attributed to the emergence of possible local electric
polarizations whose inversion symmetry is broken by
inhomogeneously distributed stacking faults. A field-induced
intermediate phase is only observed when a magnetic field is
applied perpendicular to the Ru-Ru bonds for samples with
minimal stacking faults. Less pronounced in-plane anisotropy
is found in samples with a sizable contribution from
stacking imperfections. Our findings suggest that dielectric
measurement is a sensitive probe in detecting the structural
and magnetic properties, which may be a promising tool,
especially in studying α−RuCl3 thin-film devices.
Moreover, the stacking details of RuCl3 layers strongly
affect the ground state both in the magnetic and electric
channels. Such a fragile ground state against stacking
faults needs to be overcome for realistic applications
utilizing the magnetic and/or electric properties of
Kitaev-based physics in α−RuCl3.},
cin = {JCNS-FRM-II / JCNS-2 / JCNS-4},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)JCNS-4-20201012},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 632 - Materials – Quantum, Complex and
Functional Materials (POF4-632)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-632},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000655863000002},
doi = {10.1103/PhysRevB.103.174413},
url = {https://juser.fz-juelich.de/record/892556},
}