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@ARTICLE{Pasel:893881,
      author       = {Pasel, Joachim and Schmitt, Dirk and Samsun, Remzi Can and
                      Tschauder, Andreas and Peters, Ralf},
      title        = {{T}he autothermal reforming of oxymethylenether from the
                      power-to-fuel process},
      journal      = {International journal of hydrogen energy},
      volume       = {46},
      number       = {63},
      issn         = {0360-3199},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2021-02893},
      pages        = {31984-31994},
      year         = {2021},
      abstract     = {Synthetic energy carriers that are not based on crude oil
                      or natural gas can contribute to the transcending of
                      fossil-based sources of energy in the future. A contemporary
                      example is the organic substance, oxymethylenether (OMEn),
                      which consists of hydrogen, carbon, and oxygen. It is
                      reported in the literature that OMEn suppresses the
                      formation of harmful NOx and soot and reduces CO2 emissions
                      during the combustion process in internal combustion engines
                      due to its high oxygen content. For the investigation
                      presented in this paper, the use of OMEn was transferred to
                      the autothermal reforming (ATR) process, which is normally
                      conducted using pure diesel fuel or kerosene in order to
                      produce a hydrogen-rich reformate gas to operate fuel cell
                      systems. Different mixtures of OMEn and Ultimate diesel fuel
                      were fed into Jülich's ATR 14 at a steady state. Thereby,
                      approved reaction conditions from former ATR diesel fuel
                      experiments with respect to O2/C and H2O/C molar ratios
                      (0.47 and 1.9, respectively) and temperatures of the educts
                      were applied. It was observed that the addition of OMEn to
                      Ultimate diesel fuel resulted in stable temperatures at
                      characteristic positions within ATR 14 and had a positive
                      effect on the quality of the ATR product gas (reformate).
                      For instance, the concentration of the undesired byproducts
                      ethene and benzene decreased from 800 ppmv to the range of
                      roughly 230 ppmv and from some 130 ppmv to less than 40
                      ppmv, respectively, when the mass fraction of OMEn in the
                      OMEn/Ultimate diesel mixture was increased from $0\%$ to
                      $30\%.$},
      cin          = {IEK-14},
      ddc          = {620},
      cid          = {I:(DE-Juel1)IEK-14-20191129},
      pnm          = {1232 - Power-based Fuels and Chemicals (POF4-123)},
      pid          = {G:(DE-HGF)POF4-1232},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000691826600008},
      doi          = {10.1016/j.ijhydene.2021.06.234},
      url          = {https://juser.fz-juelich.de/record/893881},
}