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| 001 | 901865 | ||
| 005 | 20220126162544.0 | ||
| 024 | 7 | _ | |a 10.1002/adma.202103755 |2 doi |
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| 100 | 1 | _ | |a Yao, Mingyue |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a A Highly Robust Ionotronic Fiber with Unprecedented Mechanomodulation of Ionic Conduction |
| 260 | _ | _ | |a Weinheim |c 2021 |b Wiley-VCH |
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| 520 | _ | _ | |a Stretchable ionic conductors are appealing for tissue-like soft electronics, yet suffer from a tardy mechanoelectric response due to their poor modulation of ionic conduction arising from intrinsic homogeneous soft chain network. Here, a highly robust ionotronic fiber is designed by synergizing ionic liquid and liquid crystal elastomer with alternate rigid mesogen units and soft chain spacers, which shows an unprecedented strain-induced ionic conductivity boost (≈103 times enhanced as stretched to 2000% strain). Such a surprisingly high enhancement is attributed to the formation of microphase-separated low-tortuosity ion-conducting nanochannels guided by strain-induced emergence of aligned smectic mesophases, thus allowing for ultrafast ion transport that resembles the role of “swimming lanes.” Intriguingly, the boosting conductivity even reverses Pouillet's Law-dictated resistance increase at certain strains, leading to unique waveform-discernible strain sensing. Moreover, the fiber retains thermal actuation properties with a maximum of 70% strain changes upon heating, and enables integrated self-perception and actuation. The findings offer a promising molecular engineering route to mechanically modulate the ion transport behavior of ionic conductors toward advanced ionotronic applications. |
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| 700 | 1 | _ | |a Feng, Xunda |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Sun, Shengtong |0 P:(DE-HGF)0 |b 3 |e Corresponding author |
| 700 | 1 | _ | |a Wu, Peiyi |0 0000-0001-7235-210X |b 4 |e Corresponding author |
| 773 | _ | _ | |a 10.1002/adma.202103755 |g p. 2103755 - |0 PERI:(DE-600)1474949-X |n 42 |p 2103755 |t Advanced materials |v 33 |y 2021 |x 1521-4095 |
| 856 | 4 | _ | |y Restricted |u https://juser.fz-juelich.de/record/901865/files/adma.202103755.pdf |
| 856 | 4 | _ | |y Published on 2021-09-03. Available in OpenAccess from 2022-09-03. |u https://juser.fz-juelich.de/record/901865/files/wu_Advanced%20Materials%20-%202021%20-%20Yao%20-%20A%20Highly%20Robust%20Ionotronic%20Fiber%20with%20Unprecedented%20Mechanomodulation%20of%20Ionic%20Conduction-Final%20draft.pdf |
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