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000904012 1001_ $$0P:(DE-HGF)0$$aXia, Rui$$b0
000904012 245__ $$aNickel Niobate Anodes for High Rate Lithium‐Ion Batteries
000904012 260__ $$aWeinheim$$bWiley-VCH$$c2022
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000904012 520__ $$aFast charging is one of the key requirements for next-generation lithium-ion batteries, however, lithium-ion diffusion rates of typical electrode materials are limited. Nanosizing of active electrode material is a common strategy to increase the effective lithium-ion diffusion transport rate, but it also decreases the volumetric energy/power density and stability of the battery. In this work, nickel niobate NiNb2O6 is demonstrated for the first time as a new intrinsic high-rate anode material for lithium-ion batteries without the requirement of realizing nano-architectures. The NiNb2O6 host crystal structure exhibits only a single type of channel for lithium-ion intercalation and can be fully lithiated with a capacity of about 244 mAh g−1 at low current densities. Interestingly, a high diffusion coefficient of 10−12 cm2 s−1 at 300 K enables fast (dis)charging at high current densities resulting in high capacities of 140 and 50 mAh g−1 for 10 and 100C respectively. The minimal volume change during lithiation is the origin of the stable reversible lithiation process in NiNb2O6 and leads to 81% capacity retention after 20 000 cycles at 100C. Finally, full cell systems against LiFePO4 and Li[Ni0.8Co0.1Mn0.1]O2 (NCM811) cathodes demonstrate the promising energy storage performance of nickel niobate anodes in practical battery devices.
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000904012 7001_ $$0P:(DE-HGF)0$$aZhao, Kangning$$b1
000904012 7001_ $$0P:(DE-Juel1)178838$$aKuo, Liang-Yin$$b2$$ufzj
000904012 7001_ $$aZhang, Lei$$b3
000904012 7001_ $$0P:(DE-HGF)0$$aCunha, Daniel M.$$b4
000904012 7001_ $$0P:(DE-HGF)0$$aWang, Yang$$b5
000904012 7001_ $$0P:(DE-HGF)0$$aHuang, Sizhao$$b6
000904012 7001_ $$0P:(DE-HGF)0$$aZheng, Jie$$b7
000904012 7001_ $$0P:(DE-HGF)0$$aBoukamp, Bernard$$b8
000904012 7001_ $$0P:(DE-Juel1)174502$$aKaghazchi, Payam$$b9$$eCorresponding author
000904012 7001_ $$0P:(DE-HGF)0$$aSun, Congli$$b10
000904012 7001_ $$00000-0001-7995-6571$$aten Elshof, Johan E.$$b11
000904012 7001_ $$0P:(DE-Juel1)174222$$aHuijben, Mark$$b12$$eCorresponding author
000904012 773__ $$0PERI:(DE-600)2594556-7$$a10.1002/aenm.202102972$$gp. 2102972 -$$n1$$p2102972 -$$tAdvanced energy materials$$v12$$x1614-6832$$y2022
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