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| 001 | 904012 | ||
| 005 | 20240711085626.0 | ||
| 024 | 7 | _ | |a 10.1002/aenm.202102972 |2 doi |
| 024 | 7 | _ | |a 1614-6832 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2021-05582 |
| 082 | _ | _ | |a 050 |
| 100 | 1 | _ | |a Xia, Rui |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Nickel Niobate Anodes for High Rate Lithium‐Ion Batteries |
| 260 | _ | _ | |a Weinheim |c 2022 |b Wiley-VCH |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Fast charging is one of the key requirements for next-generation lithium-ion batteries, however, lithium-ion diffusion rates of typical electrode materials are limited. Nanosizing of active electrode material is a common strategy to increase the effective lithium-ion diffusion transport rate, but it also decreases the volumetric energy/power density and stability of the battery. In this work, nickel niobate NiNb2O6 is demonstrated for the first time as a new intrinsic high-rate anode material for lithium-ion batteries without the requirement of realizing nano-architectures. The NiNb2O6 host crystal structure exhibits only a single type of channel for lithium-ion intercalation and can be fully lithiated with a capacity of about 244 mAh g−1 at low current densities. Interestingly, a high diffusion coefficient of 10−12 cm2 s−1 at 300 K enables fast (dis)charging at high current densities resulting in high capacities of 140 and 50 mAh g−1 for 10 and 100C respectively. The minimal volume change during lithiation is the origin of the stable reversible lithiation process in NiNb2O6 and leads to 81% capacity retention after 20 000 cycles at 100C. Finally, full cell systems against LiFePO4 and Li[Ni0.8Co0.1Mn0.1]O2 (NCM811) cathodes demonstrate the promising energy storage performance of nickel niobate anodes in practical battery devices. |
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| 700 | 1 | _ | |a Zhao, Kangning |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Kuo, Liang-Yin |0 P:(DE-Juel1)178838 |b 2 |u fzj |
| 700 | 1 | _ | |a Zhang, Lei |b 3 |
| 700 | 1 | _ | |a Cunha, Daniel M. |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Wang, Yang |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Huang, Sizhao |0 P:(DE-HGF)0 |b 6 |
| 700 | 1 | _ | |a Zheng, Jie |0 P:(DE-HGF)0 |b 7 |
| 700 | 1 | _ | |a Boukamp, Bernard |0 P:(DE-HGF)0 |b 8 |
| 700 | 1 | _ | |a Kaghazchi, Payam |0 P:(DE-Juel1)174502 |b 9 |e Corresponding author |
| 700 | 1 | _ | |a Sun, Congli |0 P:(DE-HGF)0 |b 10 |
| 700 | 1 | _ | |a ten Elshof, Johan E. |0 0000-0001-7995-6571 |b 11 |
| 700 | 1 | _ | |a Huijben, Mark |0 P:(DE-Juel1)174222 |b 12 |e Corresponding author |
| 773 | _ | _ | |a 10.1002/aenm.202102972 |g p. 2102972 - |0 PERI:(DE-600)2594556-7 |n 1 |p 2102972 - |t Advanced energy materials |v 12 |y 2022 |x 1614-6832 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/904012/files/Advanced%20Energy%20Materials%20-%202021%20-%20Xia%20-%20Nickel%20Niobate%20Anodes%20for%20High%20Rate%20Lithium%25u2010Ion%20Batteries.pdf |y OpenAccess |
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