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100 1 _ |a Deutz, Sarah
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245 _ _ |a Life-cycle assessment of an industrial direct air capture process based on temperature–vacuum swing adsorption
260 _ _ |a London
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520 _ _ |a Current climate targets require negative carbon dioxide (CO2) emissions. Direct air capture is a promising negative emission technology, but energy and material demands lead to trade-offs with indirect emissions and other environmental impacts. Here, we show by life-cycle assessment that the commercial direct air capture plants in Hinwil and Hellisheiði operated by Climeworks can already achieve negative emissions today, with carbon capture efficiencies of 85.4% and 93.1%. The climate benefits of direct air capture, however, depend strongly on the energy source. When using low-carbon energy, as in Hellisheiði, adsorbent choice and plant construction become more important, inducing up to 45 and 15 gCO2e per kilogram CO2 captured, respectively. Large-scale deployment of direct air capture for 1% of the global annual CO2 emissions would not be limited by material and energy availability. However, the current small-scale production of amines for the adsorbent would need to be scaled up by more than an order of magnitude. Other environmental impacts would increase by less than 0.057% when using wind power and by up to 0.30% for the global electricity mix forecasted for 2050. Energy source and efficiency are essential for direct air capture to enable both negative emissions and low-carbon fuels.
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700 1 _ |a Bardow, André
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773 _ _ |a 10.1038/s41560-020-00771-9
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856 4 _ |y Published on 2021-02-04. Available in OpenAccess from 2021-08-04.
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