001     905288
005     20240712113145.0
024 7 _ |a 10.1039/D1NR06435E
|2 doi
024 7 _ |a 2040-3364
|2 ISSN
024 7 _ |a 2040-3372
|2 ISSN
024 7 _ |a 2128/30300
|2 Handle
024 7 _ |a altmetric:117526502
|2 altmetric
024 7 _ |a pmid:34846412
|2 pmid
024 7 _ |a WOS:000723812900001
|2 WOS
037 _ _ |a FZJ-2022-00559
082 _ _ |a 600
100 1 _ |a Colliard-Granero, André
|0 P:(DE-Juel1)188204
|b 0
245 _ _ |a Deep learning for the automation of particle analysis in catalyst layers for polymer electrolyte fuel cells
260 _ _ |a Cambridge
|c 2022
|b RSC Publ.
336 7 _ |a article
|2 DRIVER
336 7 _ |a Output Types/Journal article
|2 DataCite
336 7 _ |a Journal Article
|b journal
|m journal
|0 PUB:(DE-HGF)16
|s 1676461577_10240
|2 PUB:(DE-HGF)
336 7 _ |a ARTICLE
|2 BibTeX
336 7 _ |a JOURNAL_ARTICLE
|2 ORCID
336 7 _ |a Journal Article
|0 0
|2 EndNote
520 _ _ |a The rapidly growing use of imaging infrastructure in the energy materials domain drives significant data accumulation in terms of their amount and complexity. The applications of routine techniques for image processing in materials research are often ad hoc, indiscriminate, and empirical, which renders the crucial task of obtaining reliable metrics for quantifications obscure. Moreover, these techniques are expensive, slow, and often involve several preprocessing steps. This paper presents a novel deep learning-based approach for the high-throughput analysis of the particle size distributions from transmission electron microscopy (TEM) images of carbon-supported catalysts for polymer electrolyte fuel cells. A dataset of 40 high-resolution TEM images at different magnification levels, from 10 to 100 nm scales, was annotated manually. This dataset was used to train the U-Net model, with the StarDist formulation for the loss function, for the nanoparticle segmentation task. StarDist reached a precision of 86%, recall of 85%, and an F1-score of 85% by training on datasets as small as thirty images. The segmentation maps outperform models reported in the literature for a similar problem, and the results on particle size analyses agree well with manual particle size measurements, albeit at a significantly lower cost.
536 _ _ |a 1231 - Electrochemistry for Hydrogen (POF4-123)
|0 G:(DE-HGF)POF4-1231
|c POF4-123
|f POF IV
|x 0
536 _ _ |a 5112 - Cross-Domain Algorithms, Tools, Methods Labs (ATMLs) and Research Groups (POF4-511)
|0 G:(DE-HGF)POF4-5112
|c POF4-511
|f POF IV
|x 1
588 _ _ |a Dataset connected to CrossRef, Journals: juser.fz-juelich.de
700 1 _ |a Batool, Mariah
|0 P:(DE-HGF)0
|b 1
700 1 _ |a Jankovic, Jasna
|0 P:(DE-HGF)0
|b 2
700 1 _ |a Jitsev, Jenia
|0 P:(DE-Juel1)158080
|b 3
|u fzj
700 1 _ |a Eikerling, Michael H.
|0 P:(DE-Juel1)178034
|b 4
700 1 _ |a Malek, Kourosh
|0 P:(DE-Juel1)181057
|b 5
|e Corresponding author
700 1 _ |a Eslamibidgoli, Mohammad Javad
|0 P:(DE-Juel1)181059
|b 6
|e Corresponding author
773 _ _ |a 10.1039/D1NR06435E
|g Vol. 14, no. 1, p. 10 - 18
|0 PERI:(DE-600)2515664-0
|n 1
|p 10 - 18
|t Nanoscale
|v 14
|y 2022
|x 2040-3364
856 4 _ |u https://juser.fz-juelich.de/record/905288/files/Invoice_INV_017301.pdf
856 4 _ |u https://juser.fz-juelich.de/record/905288/files/Nanoscale_2021.pdf
|y Published on 2021-11-24. Available in OpenAccess from 2022-11-24.
856 4 _ |u https://juser.fz-juelich.de/record/905288/files/d1nr06435e.pdf
|y Restricted
909 C O |o oai:juser.fz-juelich.de:905288
|p openaire
|p open_access
|p OpenAPC
|p driver
|p VDB
|p openCost
|p dnbdelivery
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 0
|6 P:(DE-Juel1)188204
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 3
|6 P:(DE-Juel1)158080
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 4
|6 P:(DE-Juel1)178034
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 5
|6 P:(DE-Juel1)181057
910 1 _ |a Forschungszentrum Jülich
|0 I:(DE-588b)5008462-8
|k FZJ
|b 6
|6 P:(DE-Juel1)181059
913 1 _ |a DE-HGF
|b Forschungsbereich Energie
|l Materialien und Technologien für die Energiewende (MTET)
|1 G:(DE-HGF)POF4-120
|0 G:(DE-HGF)POF4-123
|3 G:(DE-HGF)POF4
|2 G:(DE-HGF)POF4-100
|4 G:(DE-HGF)POF
|v Chemische Energieträger
|9 G:(DE-HGF)POF4-1231
|x 0
913 1 _ |a DE-HGF
|b Key Technologies
|l Engineering Digital Futures – Supercomputing, Data Management and Information Security for Knowledge and Action
|1 G:(DE-HGF)POF4-510
|0 G:(DE-HGF)POF4-511
|3 G:(DE-HGF)POF4
|2 G:(DE-HGF)POF4-500
|4 G:(DE-HGF)POF
|v Enabling Computational- & Data-Intensive Science and Engineering
|9 G:(DE-HGF)POF4-5112
|x 1
914 1 _ |y 2022
915 _ _ |a Embargoed OpenAccess
|0 StatID:(DE-HGF)0530
|2 StatID
915 _ _ |a WoS
|0 StatID:(DE-HGF)0113
|2 StatID
|b Science Citation Index Expanded
|d 2021-01-27
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0160
|2 StatID
|b Essential Science Indicators
|d 2021-01-27
915 _ _ |a National-Konsortium
|0 StatID:(DE-HGF)0430
|2 StatID
|d 2022-11-12
|w ger
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0300
|2 StatID
|b Medline
|d 2022-11-12
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0199
|2 StatID
|b Clarivate Analytics Master Journal List
|d 2022-11-12
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0150
|2 StatID
|b Web of Science Core Collection
|d 2022-11-12
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)1150
|2 StatID
|b Current Contents - Physical, Chemical and Earth Sciences
|d 2022-11-12
915 _ _ |a JCR
|0 StatID:(DE-HGF)0100
|2 StatID
|b NANOSCALE : 2021
|d 2022-11-12
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0200
|2 StatID
|b SCOPUS
|d 2022-11-12
915 _ _ |a IF >= 5
|0 StatID:(DE-HGF)9905
|2 StatID
|b NANOSCALE : 2021
|d 2022-11-12
920 _ _ |l yes
920 1 _ |0 I:(DE-Juel1)IEK-13-20190226
|k IEK-13
|l IEK-13
|x 0
920 1 _ |0 I:(DE-Juel1)JSC-20090406
|k JSC
|l Jülich Supercomputing Center
|x 1
980 1 _ |a APC
980 1 _ |a FullTexts
980 _ _ |a journal
980 _ _ |a VDB
980 _ _ |a I:(DE-Juel1)IEK-13-20190226
980 _ _ |a I:(DE-Juel1)JSC-20090406
980 _ _ |a APC
980 _ _ |a UNRESTRICTED
981 _ _ |a I:(DE-Juel1)IET-3-20190226


LibraryCollectionCLSMajorCLSMinorLanguageAuthor
Marc 21