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@ARTICLE{Basak:907457,
      author       = {Basak, Shibabrata and Tavabi, Amir H. and Dzieciol,
                      Krzysztof and Migunov, Vadim and Arszelewska, Violetta and
                      Tempel, Hermann and Kungl, Hans and Kelder, Erik M. and
                      Wagemaker, Marnix and George, Chandramohan and Mayer,
                      Joachim and Dunin-Borkowski, Rafal E. and Eichel,
                      Rüdiger-A.},
      title        = {{O}perando transmission electron microscopy of battery
                      cycling: thickness dependent breaking of {T}i{O} 2 coating
                      on {S}i/{S}i{O} 2 nanoparticles},
      journal      = {Chemical communications},
      volume       = {58},
      number       = {19},
      issn         = {0009-241X},
      address      = {Cambridge},
      publisher    = {Soc.},
      reportid     = {FZJ-2022-02049},
      pages        = {3130 - 3133},
      year         = {2022},
      abstract     = {Conformal coating of silicon (Si) anode particles is a
                      common strategy for improving their mechanical integrity, to
                      mitigate battery capacity fading due to particle volume
                      expansion, which can result in particle crumbling due to
                      lithiation induced strain and excessive solid–electrolyte
                      interface formation. Here, we use operando transmission
                      electron microscopy in an open cell to show that TiO2
                      coatings on Si/SiO2 particles undergo thickness dependent
                      rupture on battery cycling where thicker coatings crumble
                      more readily than thinner (∼5 nm) coatings, which
                      corroborates the difference in their capacities.},
      cin          = {ER-C-1 / ER-C-2 / IEK-9},
      ddc          = {540},
      cid          = {I:(DE-Juel1)ER-C-1-20170209 / I:(DE-Juel1)ER-C-2-20170209 /
                      I:(DE-Juel1)IEK-9-20110218},
      pnm          = {5351 - Platform for Correlative, In Situ and Operando
                      Characterization (POF4-535) / 5353 - Understanding the
                      Structural and Functional Behavior of Solid State Systems
                      (POF4-535) / 1223 - Batteries in Application (POF4-122) /
                      Electroscopy - Electrochemistry of All-solid-state-battery
                      Processes using Operando Electron Microscopy (892916)},
      pid          = {G:(DE-HGF)POF4-5351 / G:(DE-HGF)POF4-5353 /
                      G:(DE-HGF)POF4-1223 / G:(EU-Grant)892916},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000751912700001},
      doi          = {10.1039/D1CC07172F},
      url          = {https://juser.fz-juelich.de/record/907457},
}