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000908066 1001_ $$0P:(DE-Juel1)173990$$aLin, You-Ron$$b0
000908066 245__ $$aBoron nitride on SiC(0001)
000908066 260__ $$aCollege Park, MD$$bAPS$$c2022
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000908066 520__ $$aIn the field of van der Waals heterostructures, the twist angle between stacked two-dimensional layers has been identified to be of utmost importance for the properties of the heterostructures. In this context, we previously reported the growth of a single layer of unconventionally oriented epitaxial graphene that forms in a surfactant atmosphere [F. C. Bocquet et al., Phys. Rev. Lett. 125, 106102 (2020)]. The resulting G-R0∘ layer is aligned with the SiC lattice, and hence represents an important milestone towards high-quality twisted bilayer graphene, a frequently investigated model system in this field. Here, we focus on the surface structures obtained in the same surfactant atmosphere, but at lower preparation temperatures at which a boron nitride template layer forms on SiC(0001). In a comprehensive study based on complementary experimental and theoretical techniques, we find—in contrast to the literature—that this template layer is a hexagonal BxNy layer, but not high-quality hBN. It is aligned with the SiC lattice and gradually replaced by low-quality graphene in the 0∘ orientation of the BxNy template layer upon annealing.
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000908066 7001_ $$0P:(DE-Juel1)161374$$aFranke, Markus$$b1
000908066 7001_ $$00000-0001-7976-1344$$aParhizkar, Shayan$$b2
000908066 7001_ $$0P:(DE-Juel1)172607$$aRaths, Miriam$$b3
000908066 7001_ $$0P:(DE-HGF)0$$aWen-zhe Yu, Victor$$b4
000908066 7001_ $$0P:(DE-HGF)0$$aLee, Tien-Lin$$b5
000908066 7001_ $$aSoubatch, Serguei$$b6
000908066 7001_ $$00000-0001-8660-7230$$aBlum, Volker$$b7
000908066 7001_ $$0P:(DE-Juel1)128791$$aTautz, F. Stefan$$b8
000908066 7001_ $$0P:(DE-Juel1)128774$$aKumpf, Christian$$b9
000908066 7001_ $$0P:(DE-Juel1)167128$$aBocquet, François C.$$b10$$eCorresponding author
000908066 773__ $$0PERI:(DE-600)2898355-5$$a10.1103/PhysRevMaterials.6.064002$$gVol. 6, no. 6, p. 064002$$n6$$p064002$$tPhysical review materials$$v6$$x2475-9953$$y2022
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