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@ARTICLE{Wu:909247,
      author       = {Wu, Baolin and Chen, Chunguang and Danilov, Dmitri L. and
                      Jiang, Ming and Raijmakers, Luc H. J. and Eichel,
                      Rüdiger-A. and Notten, Peter H. L.},
      title        = {{I}nfluence of the {SEI} formation on the stability and
                      lithium diffusion in {S}i electrodes},
      journal      = {ACS omega},
      volume       = {7},
      number       = {36},
      issn         = {2470-1343},
      address      = {Washington, DC},
      publisher    = {ACS Publications},
      reportid     = {FZJ-2022-03083},
      pages        = {32740 - 32748},
      year         = {2022},
      abstract     = {Silicon (Si) is an attractive anode material for Li-ion
                      batteries (LIBs) due to its high theoretical specific
                      capacity. However, the solid–electrolyte interphase (SEI)
                      formation, caused by liquid electrolyte decomposition, often
                      befalls Si electrodes. The SEI layer is less Li-ion
                      conductive, which would significantly inhibit Li-ion
                      transport and delay the reaction kinetics. Understanding the
                      interaction between the SEI components and Li-ion diffusion
                      is crucial for further improving the cycling performance of
                      Si. Herein, different liquid electrolytes are applied to
                      investigate the induced SEI components, structures, and
                      their role in Li-ion transport. It is found that Si
                      electrodes exhibit higher discharge capacities in
                      LiClO4-based electrolytes than in LiPF6-based electrolytes.
                      This behavior suggests that a denser and more conductive SEI
                      layer is formed in LiClO4-based electrolytes. In addition, a
                      coating of a Li3PO4 artificial SEI layer on Si suppresses
                      the formation of natural SEI formation, leading to higher
                      capacity retentions. Furthermore, galvanostatic intermittent
                      titration technique (GITT) measurements are applied to
                      calculate Li-ion diffusion coefficients, which are found in
                      the range of 10–23–10–19 m2/s.},
      cin          = {IEK-9},
      ddc          = {660},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {1223 - Batteries in Application (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1223},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {36120060},
      UT           = {WOS:000855059100001},
      doi          = {10.1021/acsomega.2c04415},
      url          = {https://juser.fz-juelich.de/record/909247},
}