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@ARTICLE{Basak:909285,
author = {Basak, Shibabrata and Dzieciol, Krzysztof and Durmus, Yasin
Emre and Tempel, Hermann and Kungl, Hans and George,
Chandramohan and Mayer, Joachim and Eichel, Rüdiger-A.},
title = {{C}haracterizing battery materials and electrodes via in
situ / operando transmission electron microscopy},
journal = {Chemical Physics Reviews},
volume = {3},
number = {3},
issn = {2688-4070},
address = {[Melville, NY]},
publisher = {AIP Publishing},
reportid = {FZJ-2022-03099},
pages = {031303-1 - 031303-21},
year = {2022},
abstract = {In situ transmission electron microscopy (TEM) research has
enabled better understanding of various battery chemistries
(Li-ion, Li–S, metal–O2, Li, and Na metal based, etc.),
which fueled substantial developments in battery
technologies. In this review, we highlight some of the
recent developments shedding new light on battery materials
and electrochemistry via TEM. Studying battery electrode
processes depending on the type of electrolytes used and the
nature of electrode–electrolyte interfaces established
upon battery cycling conditions is key to further adoption
of battery technologies. To this end, in situ/operando TEM
methodologies would require accommodating alongside
correlation microscopy tools to predict battery interface
evolution, reactivity, and stability, for which the use of
x-ray computed tomography and image process via machine
learning providing complementary information is highlighted.
Such combined approaches have potential to translate
TEM-based battery results into more direct macroscopic
relevance for the optimization of real-world batteries.},
cin = {IEK-9 / ER-C-2},
ddc = {540},
cid = {I:(DE-Juel1)IEK-9-20110218 / I:(DE-Juel1)ER-C-2-20170209},
pnm = {1223 - Batteries in Application (POF4-122) / 5351 -
Platform for Correlative, In Situ and Operando
Characterization (POF4-535) / 5353 - Understanding the
Structural and Functional Behavior of Solid State Systems
(POF4-535) / Electroscopy - Electrochemistry of
All-solid-state-battery Processes using Operando Electron
Microscopy (892916)},
pid = {G:(DE-HGF)POF4-1223 / G:(DE-HGF)POF4-5351 /
G:(DE-HGF)POF4-5353 / G:(EU-Grant)892916},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001098623400003},
doi = {10.1063/5.0075430},
url = {https://juser.fz-juelich.de/record/909285},
}