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@ARTICLE{Lu:909380,
      author       = {Lu, Xin and Tsai, Chih-Long and Yu, Shicheng and He,
                      Hongying and Camara, Osmane and Tempel, Hermann and Liu,
                      Zigeng and Windmüller, Anna and Alekseev, Evgeny and Basak,
                      Shibabrata and Lu, Li and Eichel, Rüdiger-A. and Kungl,
                      Hans},
      title        = {{L}ithium {P}hosphosulfide {E}lectrolytes for
                      {S}olid-{S}tate {B}atteries: {P}art {I}},
      journal      = {Functional materials letters},
      volume       = {15},
      number       = {5},
      issn         = {1793-6047},
      address      = {Singapore ˜[u.a.]œ},
      publisher    = {World Scientific},
      reportid     = {FZJ-2022-03168},
      pages        = {2240001},
      year         = {2022},
      abstract     = {A high performance and stable Li-ion conductive solid
                      electrolyte is one of the key components for the future
                      all-solid-state batteries with metallic lithium anodes.
                      Phosphate, oxide and phosphosulfide-based inorganic solid
                      electrolytes are currently under development. High ambient
                      temperature Li-ion conductivities amounting up to 10−2 S
                      cm−1 for the best performing electrolytes distinguish the
                      phosphosulfides from the other material systems. Part I of
                      the review starts with the motivation and background for the
                      development of Li-phosphosulfide electrolytes followed by an
                      overview of four different types of phosphosulfide
                      electrolytes; the Li–P–S, thio-LiSICon, LGPS and the
                      Argyrodite-type electrolytes. The core of part I is
                      concerned with a detailed discussion of the phosphosulfide
                      electrolyte types that have been under investigation already
                      for a long time, the Li–P–S and the LiSICon. There is a
                      multiplicity of different compositions within each of these
                      types. The idea behind the outline of these sections is to
                      point out the relations and differences between the
                      different materials with respect to their chemistry related
                      to the phase diagrams. Patterns for the relations among the
                      materials identified in the phase diagrams are the base for
                      a discussion of structure, processing and Li-ion
                      conductivity within separate sections for each type and
                      resulting in intra-type comparisons. The follow up part II
                      will continue with a treatment of the more recently
                      developed LGPS and Argyrodite-type electrolytes tracking the
                      same concept, before addressing an inter-type comparison of
                      ambient temperature Li-ion conductivities and the
                      electrochemical stability of the electrolytes vs. metallic
                      lithium. A final section in part II summarizes conclusions
                      and provides perspectives for future research on Li-ion
                      conductive phosphosulfide electrolytes.},
      cin          = {IEK-9},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {1223 - Batteries in Application (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1223},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000848584400001},
      doi          = {10.1142/S179360472240001X},
      url          = {https://juser.fz-juelich.de/record/909380},
}