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@ARTICLE{Woolley:916804,
      author       = {Woolley, Henry M. and Vargas-Barbosa, Nella M.},
      title        = {{H}ybrid solid electrolyte-liquid electrolyte systems for
                      (almost) solid-state batteries: {W}hy, how, and where to?},
      journal      = {Journal of materials chemistry / A},
      volume       = {11},
      number       = {3},
      issn         = {2050-7488},
      address      = {London ˜[u.a.]œ},
      publisher    = {RSC},
      reportid     = {FZJ-2023-00107},
      pages        = {1083-1097},
      year         = {2023},
      abstract     = {All-solid-state batteries (SSBs) offer an alternative to
                      current state of the art lithium-ion batteries, promising
                      improved safety and higher energy densities due to the
                      incorporation of non-flammable solid electrolytes and Li
                      metal as an anode material. Despite this, SSBs face numerous
                      issues, including the tendency for the solid electrolytes to
                      decompose upon contact with anode and cathode materials as
                      well as during cycling. In addition, poor particle on
                      particle contact can result in sluggish transport of lithium
                      ions to and from the solid electrolytes. One potential
                      solution is by combining the solid electrolyte with a liquid
                      electrolyte to form a hybrid solid–liquid electrolyte
                      system. By using a liquid electrolyte with a wide
                      electrochemical stability window and good wetting properties
                      some of the problems with solid electrolytes in SSBs may be
                      overcome. However, due to the reactive nature of solid
                      electrolytes, a new interphase known as the solid liquid
                      electrolyte interphase (SLEI) forms. This SLEI may be
                      resistive and therefore increase the total impedance of the
                      cell, thus making certain liquid/solid electrolyte
                      combinations unsuitable for use in ASSBs. In this review we
                      discuss the recent history of these systems, look into the
                      ionic transport model and focus on how the chemical
                      stability of the solid electrolyte with respect to the
                      liquid electrolyte is a vital factor in the formation of a
                      stable SLEI. In the case of salt-in-solvent systems the
                      stability of the solid electrolyte is driven by the chemical
                      nature of the solvent, therefore we also discuss what
                      solvent properties-such as dielectric constant or donor
                      number-may have an effect on the degree of decomposition of
                      the solid electrolyte used.},
      cin          = {IEK-12},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / 1222 -
                      Components and Cells (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(DE-HGF)POF4-1222},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000901486000001},
      doi          = {10.1039/D2TA02179J},
      url          = {https://juser.fz-juelich.de/record/916804},
}